Scintillators,
as spectral and energy transformers, are essential for X-ray imaging
applications. However, their current disadvantages, including high-temperature
sintering and generation of agglomerated powders or large bulk crystals,
may not meet the increasing demands of low cost, nontoxicity, and
flexible radiation detection. Thus, improved perovskite scintillators
are developed in this research. A hybrid perovskite ((C8H17NH3)2SnBr4), which
is nontoxic, lead-free, and organic–inorganic, is developed
as a scintillator with good emission performance and radioluminescence
intensity. These perovskite scintillators are synthesized at low temperatures
in an aqueous acid solution, through which they generate a near-unity
photoluminescence quantum yield of 98% with the excitation of ultraviolet
light. As far as we know, this work is the first to show that the
two-dimensional (2D) (C8H17NH3)2SnBr4 perovskite scintillator films prepared by
coating a polymer layer can be applied to an X-ray imaging system.
The results demonstrate that the low cost X-ray imaging device with
good resolution and performance benefits dramatically from this lead-free
organic–inorganic hybrid perovskite film. Therefore, this 2D-layered
(C8H17NH3)2SnBr4 perovskite scintillator may be a high potential candidate for scintillating
material for X-ray imaging techniques.