Abstract:A review of the current state of knowledge on the effects of radiation on concrete in nuclear power production applications is presented. Emphasis is placed on the effects of radiation damage, as reflected by changes in engineering properties of concrete, in the evaluation of the long-term operation and for plant life or aging management of nuclear power plants (NPPs) in Japan, Spain, and the United States. National issues and concerns are described for Japan and the United States followed by a discussion of t… Show more
“…The obtained neutron fluence value is in accordance with the limit value for the fast neutrons proposed by United States Nuclear Regulatory Committee, (US Nuclear Regulatory Commission, 2016), and the new reference value proposed in Japan for the fast neutron fluence, (Maruyama et al, 2017), which is equal to 1•10 19 n/cm 2 . Here it should be noted that the biological shield of some PWR reactors which are used in the USA and Japan is not only a shielding structure but also a load-bearing structure, (Rosseel et al, 2016). Therefore, its damage or displacement may result in serious consequences.…”
The numerical approach for the coupled damage-creep modeling of concrete biological shield, which combines the current and the past knowledge regarding the effects of irradiation and temperature on concrete with the real measured and calculated neutron fluence and temperature distribution for VVER-440/213 reactors, is described in detail in this study. The proposed approach takes into account the real structural geometry as well as the real neutron fluence and temperature distribution and the latest knowledge about the effect of irradiation and temperature on concrete strength and stiffness. The radiation induced volumetric expansion and the thermal expansion of concrete are modeled. According to the results of the numerical simulation, the analyzed structure reaches critical damage within the time interval from 10.00 to 35.25 years of normal operation. The damage of the concrete biological shield of the VVER reactor will not affect the load-bearing function of the containment building, since the biological shield is self-bearing. The shielding properties of the biological shield may be reduced due to the appearance of the radial cracks, however, the concrete wall, which is situated right behind the biological shield, will ensure the necessary shielding. Therefore, the concrete biological shield of the VVER reactors can be considered as sacrificial structure and can be damaged without significant consequences. However, this study implies the importance of capability to predict the behavior of those PWR reactor biological shields which serve both the load-bearing and shielding purposes.
“…The obtained neutron fluence value is in accordance with the limit value for the fast neutrons proposed by United States Nuclear Regulatory Committee, (US Nuclear Regulatory Commission, 2016), and the new reference value proposed in Japan for the fast neutron fluence, (Maruyama et al, 2017), which is equal to 1•10 19 n/cm 2 . Here it should be noted that the biological shield of some PWR reactors which are used in the USA and Japan is not only a shielding structure but also a load-bearing structure, (Rosseel et al, 2016). Therefore, its damage or displacement may result in serious consequences.…”
The numerical approach for the coupled damage-creep modeling of concrete biological shield, which combines the current and the past knowledge regarding the effects of irradiation and temperature on concrete with the real measured and calculated neutron fluence and temperature distribution for VVER-440/213 reactors, is described in detail in this study. The proposed approach takes into account the real structural geometry as well as the real neutron fluence and temperature distribution and the latest knowledge about the effect of irradiation and temperature on concrete strength and stiffness. The radiation induced volumetric expansion and the thermal expansion of concrete are modeled. According to the results of the numerical simulation, the analyzed structure reaches critical damage within the time interval from 10.00 to 35.25 years of normal operation. The damage of the concrete biological shield of the VVER reactor will not affect the load-bearing function of the containment building, since the biological shield is self-bearing. The shielding properties of the biological shield may be reduced due to the appearance of the radial cracks, however, the concrete wall, which is situated right behind the biological shield, will ensure the necessary shielding. Therefore, the concrete biological shield of the VVER reactors can be considered as sacrificial structure and can be damaged without significant consequences. However, this study implies the importance of capability to predict the behavior of those PWR reactor biological shields which serve both the load-bearing and shielding purposes.
“…While deteriorations of concrete structures have been extensively researched in civil engineering field, there still remains the characteristic deterioration environment, i.e., irradiation, fully unexploited in NPPs (Rosseel et al 2016). Biological shielding concrete walls (in case of a pressurized water reactor; PWR) or reactor vessel support pedestals (in case of a boiling water reactor; BWR) are irradiated by neutrons and gamma rays from the reactor during operation.…”
We investigated changes in the density of natural rock minerals following high-energy electron irradiation, using the plasmon peak shift of electron energy-loss spectra and transmission electron microscopy. The target materials were the natural rock minerals α-quartz, orthoclase, anorthite, albite, biotite, muscovite, and chlorite. These crystalline minerals can be classified into three groups based on their Si-network geometries: 3-dimensional 6-member ring; 4-member ring + 6-member ring; and planar 6-member ring. The metamictization rates and changes in relative density are discussed using a phenomenological model, which we used to identify the physical parameters that describe the metamictization process as a function of the volume density of Si and Al atoms, or Si atoms alone, in the crystal structures. The relative densities following metamictization all decreased by more than a few percent, except for albite, which became denser. These results suggest that radiolysis damage causes initial compaction, then metamictization, characterized by the expansion of the Siand Al-polyhedra in the aggregate. The stability of concrete containing α-quartz, orthoclase, and anorthite should be further investigated in the light of the present results.
“…For nuclear applications, the study of irradiation effects on minerals and ceramics is motivated by two issues: (1) finding sustainable encapsulation matrix for radiological waste forms and Pu surplus, and, (2) assessing the long-term operation and the structural significance of exposing the concrete of nuclear power plant to high levels of neutron and gamma radiation, e.g., (Dubrovskii et al 1967;Kontani et al 2010;Rosseel et al 2016).…”
Neutron radiation-induced volumetric expansion (RIVE) of concrete aggregate is recognized as a major degradation mechanism causing extensive damage to concrete constituents (Hilsdorf et al. 1978;Seeberger and Hilsdorf 1982;. Nearly 400 RIVE data obtained in test-reactors on varied rock-forming minerals were collected by Denisov et al. (2012). These data were input into the Oak Ridge National Laboratory (ORNL) irradiated minerals, aggregates and concrete (IMAC) database and were reanalyzed in order to develop a general empirical model for minerals RIVE and interpret the susceptibility of silicates toward expansion. The empirical models best regression coefficient (r 2 ≈ 0.95) is obtained by combining two different modeling techniques: (1) an interpolation-like model based on the relative distance to existing data points, and, (2) a nonlinear regression model assuming varied mathematical forms to describe RIVE as a function of the neutron fluence 3 and the average irradiation temperature. The susceptibility to develop irradiation-induced expansion greatly varies with the nature of minerals. Silicates, i.e., [SiO 4 ] 4-bearing minerals show a wide range of maximum RIVEs, from a few percents to what appears as a bounding value of 17.8% for quartz. The maximum RIVE of varied silicates appears to be governed, macroscopically, by three parameters: (1) Primarily, the dimensionality of silicate polymerization (DOSP), (2) the relative number of Si-O bond per unit cell, and, (3) the relative bonding energy (RBE) of the unit cell.
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