Ferromagnetic resonance and magneto-optic Kerr effect (MOKE) techniques are employed to unravel the nature of ‘in-plane’ (IP) magnetic anisotropy and magnetization reversal (MR) processes in magnetron-sputtered 100 nm Co2Fe0.5Ti0.5Si (CFTS) thin films, deposited (and subsequently annealed) at different substrate temperatures (Ts) ranging from 200°C to 550°C. By varying TS, the CFTS films are produced with different amounts of anti-site (AS) atomic disorder. Irrespective of the degree of AS disorder, the IP uniaxial magnetic anisotropy (UMA) is prevalent in all the CFTS films. The TS450 and TS500 films, deposited at TS = 450 oC and 500 oC, stand out as they have (i) the least AS disorder, (ii) lowest value (α = 0.0055) of the Gilbert damping constant, (iii) high saturation magnetization (≅ 770 ) at 300 K, (iv) UMA
at300 K, (v) spin-wave stiffness (0 ≅ 175Å2 and, as in other CFTS films,the electron-magnon interaction is primarily responsible for the thermal renormalization of.Furthermore, in the TS450 and TS500 films, MOKE hysteresis loops at various angles ()