Regulation characteristics of oxide generation and formaldehyde removal by using volume DBD reactor

Abstract

Discharge plasmas in air can be accompanied by ultraviolet (UV) radiation and electron impact, which can produce large numbers of reactive species such as hydroxyl radical (OH•), oxygen radical (O•), ozone (O 3), and nitrogen oxides (NO x), etc. The composition and dosage of reactive species usually play an important role in the case of volatile organic compounds (VOCs) treatment with the discharge plasmas. In this paper, we propose a volume discharge setup used to purify formaldehyde in air, which is configured by a plate-to-plate dielectric barrier discharge (DBD) channel and excited by an AC high voltage source. The results show that the relative spectral-intensity from DBD cell without formaldehyde is stronger than the case with formaldehyde. The energy efficiency ratios (EERs) of both oxides yield and formaldehyde removal can be regulated by the gas flow velocity in DBD channel, and the most desirable processing effect is the gas flow velocity within the range from 2.50 to 3.33 m s −1. Moreover, the EERs of both the generated dosages of oxides (O 3 and NO 2) and the amount of removed formaldehyde can also be regulated by both of the applied voltage and power density loaded on the DBD cell. Additionally, the EERs of both oxides generation and formaldehyde removal present as a function of normal distribution with increasing the applied power density, and the peak of the function is appeared in the range from 273.5 to 400.0 W l −1. This work clearly demonstrates the regulation characteristic of both the formaldehyde removal and oxides yield by using volume DBD, and it is helpful in the applications of VOCs removal by using discharge plasma.

Characteristics of water volatilization and oxides generation by using positive and negative corona

“…There are many reactive species in the discharge area, such as ultraviolet (UV), energetic electrons, hydroxyl radical (OH), oxygen radical (O), ozone (O 3 ), and nitrogen oxides (NO x ), and so on. Therefore, discharge plasmas have high potential application value in the environmental remediation [3,4], advanced materials [5][6][7], life and health [8,9], low-carbon energy [10,11], advanced manufacturing [12], agricultural production [13,14], and other fields [15][16][17].…”

Preparation of graphene-based catalysts and combined DBD reactor for VOC degradation

“…with the output voltage of 12 kV and ow rate of 275 L/h, O 3 concentration produced by SDBD was about 3787.43 ppm, and that produced by DDBD was about 2144.47 ppm. For the constant SED, the transformation rate of O 3 increased with the build-up of output voltage (Fig.4a), indicating that part of O 3 generated by the plasma device was involved in the degradation of VOCs, while some part of O 3 got transformed and degraded(Mao et al, 2017;Chen et al, 2018). The higher the benzene series concentration, the more O 3 consumption.…”