single, multiple, or broadband frequency of the electromagnetic spectrum. The ultrahigh light absorption is obtained due to an impedance match between the material and the medium. [9] Here, the electric and magnetic resonances are designed so that the bulk effective impedance is equal to the one of the free space (air or vacuum). As a result, most of the incident light is absorbed and the reflection is negligible. Salisbury [10] and Dallenbach [11] first idealized classical absorbers to operate in the microwave range of the electromagnetic spectrum. The former included a resistive layer located at a quarter wavelength from a metallic substrate while the latter consisted of a dielectric layer on top of a metallic substrate.In the past two decades, advances in nanofabrication have given rise to nanostructures with controlled geometry, recently inspiring the design of metamaterials and metasurfaces for superabsorbers. [12] With the flexibility of tuning nanostructures' geometry and periodicity, such absorbers have been demonstrated in the visible, [13,14] near-infrared (NIR), [15] mid-infrared (MIR), [16] and far-infrared (FIR) [17,18] frequency ranges, proving to be a powerful approach for producing optical responses that are not feasible by any conventional material. However, the cost of the current fabrication methods limits their commercial applications. For instance, metasurfaces consisting of arrays of nanostructures on a dielectric surface are difficult to manufacture through physical deposition approaches in large scale even by using state-of-the-art bottomup nanolithography methods.To overcome the scalability constraints of the fabrication methods currently implemented for metasurfaces, the use of thin films in superabsorbers has been explored for a broad range of the spectrum, extending from visible to the FIR. [19][20][21][22][23][24][25][26][27][28] The Dallenbach configuration provides significant benefits regarding the fabrication of ultrathin, planar, omnidirectional, and polarization independent structures with very high absorption. Recently, it was reported that more than 98% of the normally incident light could be absorbed in an ultrathin layer of Ge on top of Ag at a wavelength (λ) of 625 nm, decreasing to 80% for incident angles up to 66° for both polarizations. [21] In addition, highly doped Si has been used as a metallic-like substrate under a thin Ge layer to absorb light in the MIR, where the doping concentration in Si was the knob to engineer its Superabsorbers based on metasurfaces have recently enabled the control of light at the nanoscale in unprecedented ways. Nevertheless, the sub-wavelength features needed to modify the absorption band usually require complex fabrication methods, such as electron-beam lithography. To overcome the scalability limitations associated with the fabrication of metallic nanostructures, engineering the optical response of superabsorbers by metal alloying is proposed, instead of tuning the geometry/size of the nanoscale building blocks. The superior performance...