2008
DOI: 10.1063/1.2912527
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Random lasers with coherent feedback from highly transparent polymer films embedded with silver nanoparticles

Abstract: We report on observations of random lasers with coherent feedback in highly transparent polymer films embedded with silver nanoparticles. The hybrid materials were fabricated via in situ synthesis method, through which silver nanoparticles were precipitated by thermal treatment. Sharp peaks with linewidth ϳ0.5 nm were observed to emerge on the broad emission background when the pump energy reached a threshold, together with unidirectional laser irradiation. Random lasers with coherent feedback induced by silve… Show more

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Cited by 139 publications
(116 citation statements)
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References 17 publications
(19 reference statements)
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“…RLs using Ag NPs as responsible for enhanced emission was reported before with poly(methylmethacrylate)-PMMA-as the host medium 13 or other polymers, 33,34 whereby even in the weakly scattering regime arising from the NPs smaller size and crosssection, coherent RL emission has been observed. 34 In the present case, the Ag NPs were introduced in the BC membrane as described in Sec. II.…”
Section: Resultsmentioning
confidence: 99%
“…RLs using Ag NPs as responsible for enhanced emission was reported before with poly(methylmethacrylate)-PMMA-as the host medium 13 or other polymers, 33,34 whereby even in the weakly scattering regime arising from the NPs smaller size and crosssection, coherent RL emission has been observed. 34 In the present case, the Ag NPs were introduced in the BC membrane as described in Sec. II.…”
Section: Resultsmentioning
confidence: 99%
“…Several authors have demonstrated that metal-nanoparticles dye random laser systems not only operate better than the dielectric based random lasers, but that they also work at extremely weak scattering strengths, as a result of the highly localized optical modes due to surface plasmon resonance (SPR) [37]. Moreover the lasing properties were dramatically improved when the SPR or the 'scattering resonance' wavelength of the metal particles overlapped the dye emission [35].…”
Section: Resultsmentioning
confidence: 99%
“…In these systems, metal nanoparticles may enhance the lasing efficiency by intensifying the scattering strength and/or the dye fluorescence by means of an enhanced localized field. Incoherent and coherent feedback have been demonstrated and related both to scattering and plasmon efficiency [34][35][36][37].…”
Section: Resultsmentioning
confidence: 99%
“…Such a situation is not achievable in formerly considered RL: in the fixed disorder case [4], the structure cannot be externally changed; while in the colloidal RL [6] the considered dielectric nano-particles, [18][19][20][21] are too light to exhibit a switchable granular behavior. Various authors also investigated RL by metallic nano-particles [22][23][24][25], however, so far, only particles with diameters of tens of nanometers were considered, which do not exhibit granular behavior because are not substantially affected by gravity. In these systems, thermal equilibrium largely limits the observable fluctuations with respect to out-of-equilibrium granulars.…”
mentioning
confidence: 99%