Projection-reduction method applied to deriving non-linear optical conductivity for an electron-impurity system

Abstract

The projection-reduction method introduced by the present authors is known to give a validated theory for optical transitions in the systems of electrons interacting with phonons. In this work, using this method, we derive the linear and first order nonlinear optical conductivites for an electron-impurity system and examine whether the expressions faithfully satisfy the quantum mechanical philosophy, in the same way as for the electron-phonon systems. The result shows that the Fermi distribution function for electrons, energy denominators, and electron-impurity coupling factors are contained properly in organized manners along with absorption of photons for each electron transition process in the final expressions. Furthermore, the result is shown to be represented properly by schematic diagrams, as in the formulation of electron-phonon interaction. Therefore, in conclusion, we claim that this method can be applied in modeling optical transitions of electrons interacting with both impurities and phonons

Nonlinear optical Hall effect of few-layered NbSe2

“…We numerically calculate nonlinear optical spin and charge Hall conductivities for few-layered NbSe 2 based on an effective TBM. In general, the 2nd order nonlinear optical spin conductivity can be given as 28,29,33,35,[73][74][75][76][77][78]…”