2012
DOI: 10.1364/ol.37.004934
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Probing molecular absorption under slow-light propagation using a photonic crystal waveguide

Abstract: High-resolution infrared absorption spectroscopy of acetylene gas is demonstrated in a dispersion-engineered photonic crystal waveguide under slow-light propagation. Experimental enhancement factors of 0.31 and 1.00 are obtained for TE and TM polarization, respectively, for group indices ranging from 1.5 to 6.7. The dependence of molecular absorption on the evanescent electric-field distribution and on the group index under structural slowlight illumination is experimentally demonstrated and confirmed by time-… Show more

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Cited by 23 publications
(15 citation statements)
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References 12 publications
(4 reference statements)
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“…This result also shows that the enhancement of the nonlinear effects reported before were a result of the experimental configuration -the pulse is injected into a finite length nonlinear media, and the nonlinear effect is measured at the output. Thus, unlike many previous claims, light-matter interactions are not enhanced in the slow/stopped light regimes, and the observed enhancements of the (linear and) nonlinear effects is unrelated to the source of the strong dispersion, be it material or structural dispersion [78,79]. An alternative experimental configuration where the absorption or nonlinearity are measured in systems with different group velocities for the same duration is expected to show the insensitivity to the group velocity we predict here.…”
Section: Scaling With the Group Velocitycontrasting
confidence: 50%
“…This result also shows that the enhancement of the nonlinear effects reported before were a result of the experimental configuration -the pulse is injected into a finite length nonlinear media, and the nonlinear effect is measured at the output. Thus, unlike many previous claims, light-matter interactions are not enhanced in the slow/stopped light regimes, and the observed enhancements of the (linear and) nonlinear effects is unrelated to the source of the strong dispersion, be it material or structural dispersion [78,79]. An alternative experimental configuration where the absorption or nonlinearity are measured in systems with different group velocities for the same duration is expected to show the insensitivity to the group velocity we predict here.…”
Section: Scaling With the Group Velocitycontrasting
confidence: 50%
“…The importance of the latter was demonstrated experimentally in absorption-type measurements 24 . Equation (1) agrees with the result of a perturbative analysis 25 .…”
Section: Resultsmentioning
confidence: 91%
“…To go around this difficulty, the fiber-optic sensors of liquids developed to date either rely on hollow-core, photonic crystal fibers (PCFs) [5][6][7][8] or involve considerable structural modifications of standard fibers. Specific forms of the latter include long-period fiber Bragg gratings for the excitation of cladding modes [9], etching or polishing fibers down to the core [10,11], tapering fibers down to few-microns diameters [12], the application of transducer coating layers [13], the fabrication of inline cavities [14], and the use of cleaved facets [15,16].…”
Section: Introductionmentioning
confidence: 99%