1969
DOI: 10.1103/physrevlett.22.4
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Pressure Shift and Broadening of Methane Line at 3.39μStudied by Laser-Saturated Molecular Absorption

Abstract: We study broadening and the anomalously small shift of a 3.39-JU rotation-vibration line of methane at millitorr pressures 0 Saturation by the laser intracavity field allows investigation of the very sharp natural linewidth, without Doppler broadening. Two lasers were independently locked to this transition with an offset of less than ±1 kHz, a reproducibility of ±1 x 10 u .

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Cited by 343 publications
(56 citation statements)
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“…If the frequency of the reference laser is sufficiently close to the frequency of the target laser, the two lasers may be heterodyned on a photodetector and the resulting beat note can be used to stabilize the target laser. 1 However, this is only practical up to a certain frequency difference due to the bandwidth of the photodetector.…”
Section: Introductionmentioning
confidence: 99%
“…If the frequency of the reference laser is sufficiently close to the frequency of the target laser, the two lasers may be heterodyned on a photodetector and the resulting beat note can be used to stabilize the target laser. 1 However, this is only practical up to a certain frequency difference due to the bandwidth of the photodetector.…”
Section: Introductionmentioning
confidence: 99%
“…From here A mn ≃ 4 Hza and it is only small part of all spontaneous relaxation of m-term (without collisions) as the last is ν m | P =0 ≃ 100 Hza [37].…”
Section: Radiationmentioning
confidence: 99%
“…One method that has been particularly effective is laser-saturated absorption spectroscopy developed by J. L. Hall [76,77], Schawlow [78], Hansch [78], and others [79,80,[81][82][83][84]. In such a device, laser light is passed in opposite directions through, say, a CH 4 or 12 absorption cell.…”
Section: Lasersmentioning
confidence: 99%