Abstract:In the heavy-fermion system Yb 2 Pd 2 In 1−x Sn x , the interplay of crystal-field splitting, Kondo effect, and Ruderman-Kittel-Kasuya-Yosida interactions leads to complex chemical-, pressure-, and magnetic-field phase diagrams, still to be explored in full detail. By using a series of techniques, we show that even modest changes of parameters other than temperature are sufficient to induce multiple quantum-critical transitions in this highly susceptible heavy-fermion family. In particular, we show that, above… Show more
“…For R 2 T 2 X (R=Ce,Yb), the f-electrons of the rare earths can also display mixed valence behaviors [8][9][10][11][12][13] , indicating that coupling of the f-electrons to extended states can lead to the overall suppression of magnetic moments. It is expected that the interplay of strong quantum fluctuations due to the unique R 2 T 2 X lattice [13][14][15] , and as well proximity to the delocalization of the f-electrons via the Kondo effect can result in the destabilization of ordered phases, and to the formation of quantum critical points (QCPs) where the host systems are transitioning among different phases 9,13,[16][17][18] . Given this richness of behavior when the rare earth R has f-electrons, it is surprising that relatively little is known about compounds from this family where R=La,Lu,Y , where there are no valence f-electrons.…”
We report here the properties of single crystals of La2Ni2In. Electrical resistivity and specific heat measurements concur with the results of Density Functional Theory (DFT) calculations, finding that La2Ni2In is a weakly correlated metal, where the Ni magnetism is almost completely quenched, leaving only a weak Stoner enhancement of the density of states. Superconductivity is observed at temperatures below 0.9 K. A detailed analysis of the field and temperature dependencies of the resistivity, magnetic susceptibility, and specific heat at the lowest temperatures reveals that La2Ni2In is a dirty type-II superconductor with likely s-wave gap symmetry. Nanoclusters of ferromagnetic inclusions significantly affect the subgap states resulting in a non-exponential temperature dependence of the specific heat C(T ) at T Tc.
“…For R 2 T 2 X (R=Ce,Yb), the f-electrons of the rare earths can also display mixed valence behaviors [8][9][10][11][12][13] , indicating that coupling of the f-electrons to extended states can lead to the overall suppression of magnetic moments. It is expected that the interplay of strong quantum fluctuations due to the unique R 2 T 2 X lattice [13][14][15] , and as well proximity to the delocalization of the f-electrons via the Kondo effect can result in the destabilization of ordered phases, and to the formation of quantum critical points (QCPs) where the host systems are transitioning among different phases 9,13,[16][17][18] . Given this richness of behavior when the rare earth R has f-electrons, it is surprising that relatively little is known about compounds from this family where R=La,Lu,Y , where there are no valence f-electrons.…”
We report here the properties of single crystals of La2Ni2In. Electrical resistivity and specific heat measurements concur with the results of Density Functional Theory (DFT) calculations, finding that La2Ni2In is a weakly correlated metal, where the Ni magnetism is almost completely quenched, leaving only a weak Stoner enhancement of the density of states. Superconductivity is observed at temperatures below 0.9 K. A detailed analysis of the field and temperature dependencies of the resistivity, magnetic susceptibility, and specific heat at the lowest temperatures reveals that La2Ni2In is a dirty type-II superconductor with likely s-wave gap symmetry. Nanoclusters of ferromagnetic inclusions significantly affect the subgap states resulting in a non-exponential temperature dependence of the specific heat C(T ) at T Tc.
Pressure, together with temperature, electric, and magnetic fields, alters the system and allows for the investigation of the fundamental properties of matter. Under applied pressure, the interatomic distances shrink, which modifies the interactions between atoms and may lead to the appearance of new (sometimes exotic) physical properties, such as pressure-induced phase transitions; quantum critical points; new structural, magnetic, and/or superconducting states; and changes of the temperature evolution and symmetry of the order parameters. Muon-spin rotation/relaxation ([Formula: see text]SR) has proven to be a powerful technique in elucidating the magnetic and superconducting responses of various materials under extreme conditions. At present, [Formula: see text]SR experiments may be performed in high magnetic field up to [Formula: see text] T, temperatures down to [Formula: see text]–15 mK, and hydrostatic pressure up to [Formula: see text] GPa. In this Perspective, the requirements for [Formula: see text]SR experiments under pressure, the existing high-pressure muon facility at the Paul Scherrer Institute (Switzerland), and selected experimental results obtained by [Formula: see text]SR under pressure are discussed.
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