communication, [4] environmental monitoring, [5] and wearable and neuromorphic computing. [6] This will also have an impact on the internet of things (IoT) where smart objects are wirelessly connected to interact with the environment and the human body. [7] The high-performing electronic devices made of compliant materials can add new capabilities in terms of highspeed communications, efficient image sensing, and so on. [4c,8] For example, the transmission rate, the transmission capacity, and the efficiency of wireless communication could significantly be enhanced if a single photodetector (PD) device could operate under wide spectra with low power consumption and latency. Furthermore, the demands for wide spectral switches [9] or memory storage [10] could be satisfied from the single PD. However, the studies so far have primarily focused on the development and characterization of high-performance flexible PDs under certain wavelength (i.e., UV, [1b,10,11] visible, [12] or NIR [13] spectrum). Recently, there have been few attempts to develop ultrafast and conformable broadband PDs. [8b,14] Among these, the heterostructures based on 2D materials and perovskites have shown potential to expand the working wavelength of PDs. [14] This is owing to their direct bandgap and large absorption coefficient. [15] Specifically, perovskites have garnered more interest for optoelectronic applications as they are solution processable and their fabrication cost is low. However, due to low mobility (≈1-10 cm 2 Vs) [16] and poor stability, [17] their performance metrics (e.g., responsivity [R] and specific detectivity [D*])) for PDs are modest. The poor stability in ambient conditions is attributed to the adsorption of water and oxygen molecules which greatly accelerate the degradation of the perovskite photosensitive layer. [15a] Efforts are ongoing to enhance the stability of perovskite-based devices exploring different encapsulations, but low intrinsic mobilities will still be a challenge. Thus, the efforts to develop next generation of flexible and high-performing PDs, with wide spectral sensitivity and robust fabrication route, are still on.In the above context, the nanostructures and thin films of inorganic compound semiconductors such as gallium arsenide (GaAs) have shown considerable potential for optoelectronic Nano/microstructures of compound semiconductors such as gallium arsenide (GaAs) demonstrate enormous potential for advanced photonic technologies as they provide realistic means for miniaturization of optoelectronic devices that feature better performance and low power consumption. However, intimately integrating them onto flexible substrates is challenging and restricts their use in the next generation of applications such as wearables and soft robotics. Herein, printed arrays of well-defined and laterally aligned semi-insulating (undoped) and doped GaAs microstructures are presented to develop high-performance flexible broadband photodetectors. The direct roll transfer printed GaAs microstructures-based ph...