Photon Drag Currents and Terahertz Generation in α-Sn/Ge Quantum Wells

Abstract

We have fabricated α-Sn/Ge quantum well heterostructures by sandwiching nano-films of α-Sn between Ge nanolayers. The samples were grown via e-beam deposition and characterized by Raman spectroscopy, atomic force microscopy, temperature dependence of electrical resistivity and THz time-resolved spectroscopy. We have established the presence of α-Sn phase in the polycrystalline layers together with a high electron mobility μ = 2500 ± 100 cm2 V−1 s−1. Here, the temperature behavior of the resistivity in a magnetic field is distinct from the semiconducting films and three-dimensional Dirac semimetals, which is consistent with the presence of linear two-dimensional electronic dispersion arising from the mutually inverted band structure at the α-Sn/Ge interface. As a result, the α-Sn/Ge interfaces of the quantum wells have topologically non-trivial electronic states. From THz time-resolved spectroscopy, we have discovered unusual photocurrent and THz radiation generation. The mechanisms for this process are significantly different from ambipolar diffusion currents that are responsible for THz generation in semiconducting thin films, e.g., Ge. Moreover, the THz generation in α-Sn/Ge quantum wells is almost an order of magnitude greater than that found in Ge. The substantial strength of the THz radiation emission and its polarization dependence may be explained by the photon drag current. The large amplitude of this current is a clear signature of the formation of conducting channels with high electron mobility, which are topologically protected.

Reproducible Preparation of Thin Graphene Films Using a Green and Efficient Liquid-Phase Exfoliation Method for Applications in Photovoltaics

“…Additionally, their suitability as photodetectors due to high responsivity, rapid response times, and a broad spectral range is noteworthy [44][45][46][47][48]. Graphene nanosheets also excel as saturable absorbers in mode-locked lasers, opening avenues for generating ultrashort pulses in the femtosecond regime [49,50]. Moreover, their pronounced interaction with light in the IR region positions them as promising materials for infrared sensors [51].…”