2021
DOI: 10.1021/acsami.1c10990
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Organic/Inorganic Hybrid Boosting Energy Harvesting Based on the Photothermoelectric Effect

Abstract: Attracted by the capability of light to heat and electricity conversion, the photothermoelectric (PTE) effect has drawn great attention in the field of energy conversion and self-powered electronics. However, it still requires effective strategies to convert electricity from light based on the corresponding photothermoelectric generator. Herein, considering the broad photoresponse and large Seebeck effect of tellurium nanowires (Te NWs) as well as the high electrical conductivity of poly­(3,4-ethylenedioxythio… Show more

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Cited by 33 publications
(40 citation statements)
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“…In general, the construction of composite materials relies on the high σ or high S advantage of each component to overcome their respective defects to achieve the improvement of PF . 6 This means that the introduction of CQDs can effectively improve the TE performances of PEDOT:PSS under light illumination, rather than through a compromise. Additionally, carrier concentration ( n ) and mobility ( μ ) were evaluated by the Hall effect measurement for the as-fabricated films.…”
Section: Resultsmentioning
confidence: 99%
“…In general, the construction of composite materials relies on the high σ or high S advantage of each component to overcome their respective defects to achieve the improvement of PF . 6 This means that the introduction of CQDs can effectively improve the TE performances of PEDOT:PSS under light illumination, rather than through a compromise. Additionally, carrier concentration ( n ) and mobility ( μ ) were evaluated by the Hall effect measurement for the as-fabricated films.…”
Section: Resultsmentioning
confidence: 99%
“…When the black silicon light absorber was assembled with thermoelectric modules for photo‐thermoelectric generation, it could achieve a steady voltage of ≈64 mV (Figure 7f) under AM 1.5 G illumination, which showed a performance rise rate of 28% compared with the former work. To further simplify the photo‐thermoelectric device, Liu and his colleagues [ 118 ] integrated the light absorber with thermoelectric material into one device for photo‐thermoelectric power generation. As‐prepared poly (3,4‐ethylenedioxythiophene): poly(styrenesulfonate)/Te nanowires (PEDOT: PSS/Te NW) can be seen in Figure 7g.…”
Section: Solar‐driven Photothermal Applicationsmentioning
confidence: 99%
“…i) Photo-thermoelectric conversion results for different Te NW content of PEDOT:PSS/ Te NW films. (g-i) Reproduced with permission [118]. Copyright 2021, American Chemical Society.…”
mentioning
confidence: 99%
“…The first type is so-called homogeneous synchronous PTEGs, in which the photothermal (PT) and TE conversions can be performed almost simultaneously, since the heat required for the TE conversion comes from the PT effects of the TE materials themselves or the introduced PT fillers. The design of this structure can avoid the energy waste caused by the interfacial thermal resistance on the contact surfaces of the PT and TE layers. For example, Jin et al wrapped polypyrrole (PPy) on helical carbon nanotubes to improve the PT conversion capability of PPy and thus optimize its photo-thermoelectric property, and eventually, the PTEGs constructed with this composite have fast response and excellent output stability, making them possible to be applied to delayed control systems . However, the output performance of such PTEGs is always poor because few materials have both excellent PT and TE properties, and the introduction of fillers with excellent PT properties can enhance the PT conversion capacity of composite materials to some extent, but at the same time, their poor TE properties will affect the overall TE conversion capacity of the composites.…”
Section: Introductionmentioning
confidence: 99%