Abstract:Photorefractive effects are, for the first time to our knowledge, observed in single-domain tetragonal BaTiO3 fibers fabricated by the laser pedestal method. The diameter and length of the fiber are 250 μm and 2 mm, respectively. The photorefractivity is confirmed both by beam amplification through two-wave mixing and holographic image storage.
“…12 It is also used in phase conjugation and image reconstruction. 8 Organic molecules containing conjugate systems have some advantages over inorganic materials because of the possibility of highly enhanced electronic nonlinear optical polarization responses. The basic structure of organic NLO materials is based on the π bond system; 13 due to the overlap of π orbitals, delocalization of electronic charge distribution leads to a high mobility of the electron density.…”
Section: Introductionmentioning
confidence: 99%
“…The search for new nonlinear optical (NLO) materials has been increased in the last few decades because of their potential applications in optical modulation, second-harmonic generation (SHG), optical signal processing, optical switching, optical data storage devices, etc . It is also used in phase conjugation and image reconstruction . Organic molecules containing conjugate systems have some advantages over inorganic materials because of the possibility of highly enhanced electronic nonlinear optical polarization responses.…”
Nowadays more attention has been paid to the growth of organic nonlinear optical single crystals due to their high nonlinear optical efficiency and fairly good optical damage threshold comparable to that of inorganic counterparts. The organic nonlinear optical single crystals of benzimidazole (BMZ) grown by the slow evaporation solution growth technique (SEST) and the vertical Bridgman technique (VBT) were characterized, and their results have been compared. Characterization has been made by high-resolution X-ray diffractometry (HRXRD), Fourier transform infrared (FTIR), laser damage threshold, microhardness, and second-harmonic generation (SHG) measurement studies. The high-resolution X-ray diffraction curves (DCs) recorded by an inhouse developed multicrystal X-ray diffractometer (MCD) revealed that the crystals grown by both methods contain internal structural grain boundaries. However, VBT crystals normally contain multiple low angle (tilt angle R g 1 arc min) boundaries due to thermal stress caused during the cooling cycle by the difference in the lattice expansion coefficients of the glass tube and the crystal, whereas SEST crystals were found to contain only one very low angle (R < 1 arc min) boundary probably due to entrapment of solvent in the crystal during growth. From FTIR studies, it was found that the packing of molecules is more dense in the case of VBT-grown crystals than the case of SEST-grown crystals. From the Vicker's microhardness measurements made along the [100] direction, superior mechanical behavior is observed in VBT crystals than in SEST crystals. The mechanical behavior is correlated with their laser damage threshold values.
“…12 It is also used in phase conjugation and image reconstruction. 8 Organic molecules containing conjugate systems have some advantages over inorganic materials because of the possibility of highly enhanced electronic nonlinear optical polarization responses. The basic structure of organic NLO materials is based on the π bond system; 13 due to the overlap of π orbitals, delocalization of electronic charge distribution leads to a high mobility of the electron density.…”
Section: Introductionmentioning
confidence: 99%
“…The search for new nonlinear optical (NLO) materials has been increased in the last few decades because of their potential applications in optical modulation, second-harmonic generation (SHG), optical signal processing, optical switching, optical data storage devices, etc . It is also used in phase conjugation and image reconstruction . Organic molecules containing conjugate systems have some advantages over inorganic materials because of the possibility of highly enhanced electronic nonlinear optical polarization responses.…”
Nowadays more attention has been paid to the growth of organic nonlinear optical single crystals due to their high nonlinear optical efficiency and fairly good optical damage threshold comparable to that of inorganic counterparts. The organic nonlinear optical single crystals of benzimidazole (BMZ) grown by the slow evaporation solution growth technique (SEST) and the vertical Bridgman technique (VBT) were characterized, and their results have been compared. Characterization has been made by high-resolution X-ray diffractometry (HRXRD), Fourier transform infrared (FTIR), laser damage threshold, microhardness, and second-harmonic generation (SHG) measurement studies. The high-resolution X-ray diffraction curves (DCs) recorded by an inhouse developed multicrystal X-ray diffractometer (MCD) revealed that the crystals grown by both methods contain internal structural grain boundaries. However, VBT crystals normally contain multiple low angle (tilt angle R g 1 arc min) boundaries due to thermal stress caused during the cooling cycle by the difference in the lattice expansion coefficients of the glass tube and the crystal, whereas SEST crystals were found to contain only one very low angle (R < 1 arc min) boundary probably due to entrapment of solvent in the crystal during growth. From FTIR studies, it was found that the packing of molecules is more dense in the case of VBT-grown crystals than the case of SEST-grown crystals. From the Vicker's microhardness measurements made along the [100] direction, superior mechanical behavior is observed in VBT crystals than in SEST crystals. The mechanical behavior is correlated with their laser damage threshold values.
“…planar waveguides or optical fibres) on the basis of standard photorefractive crystals which demonstrate photorefractive properties (in particular, dynamic holographic recording and phase conjugation) in addition to traditional advantages of the waveguide structures-long length of interaction and high concentration o f light energy. And indeed, some impressive technological results were obtained recently, both on producing planar photorefractive waveguides (see the review paper by van Wood et U / 1989) and on growing of single crystal optical fibres from traditional photorefractive crystals of SBN (Hesselink and Redfield 1988), LiNbO, (Yoshinaga et a/ 1990) and BaTiO, (Ito et al 1992).…”
The main suggestions in practical applications of dynamic photorefractive holographic recording for interferometry, processing of 2D pictures, operations with laser beams, and holographic memory systems are reviewed. Specific photorefractive techniques underlying these applications, and in particular, methods of continous and nondestructive hologram reconstruction, nonlinearities in recording mechanisms, and basic limitations due to geometrical factors, Bragg regime of diffraction, and optical noise are considered in detail. The paper is preceded by two introductory sections devoted to fundamentals of dynamic holography and phase conjugation in volume media, and to specific features of' recording and reconstruction of the photorefractive holograms.
“…Doped and undoped fibres of most optical materials may be grown for a wide range of potential applications in which their small size makes them compatible with miniature solid-state and diode lasers. These include such diverse topics as laser media and amplifiers [5], phase conjugation and image processing [6], sensing [7], high power optical beam delivery [8] and polarizers utilizing gradient index (GRIN) fibres [9].…”
a-axis fibres of lithium niobate produced by laser heated miniature pedestal growth can possess transverse and longitudinal birefringence variations due to faceted growth. When used for second harmonic generation, these characteristics cause conversion efficiencies to be two to three orders of magnitude smaller than predicted and the phasematchable lengths and apertures to be short. Second harmonic generation and associated birefringence mapping are shown to be sensitive indicators of their uniformity.
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