Abstract:A level set approach was adopted in numerical simulation of interphase mass transfer from a deformable drop moving in a continuous immiscible liquid, and the simulation results on Marangoni effect were presented with respect to three experimental runs in the methyl isobutyl ketone-acetic acid-water system. Experiments showed that when the solute concentration was sufficiently high, the Marangoni effect would occur with the interphase mass transfer enhanced. Numerical results indicated that the masstransfer coe… Show more
“…7 a and 7 b. The simulated results reported by Wang et al [33] overestimated significantly compared with the experimental ones, as listed in Tab. 3.…”
Section: Mass Transfer Coefficientscontrasting
confidence: 49%
“…(7). The involved coefficients [33] were given as a = -0.475 and b = 0.06 for Case 1, and a = -0.74 and b = 0.14 for Case 2. …”
The level set method is combined with the concentration transformation method to solve the interphase mass transfer process. However, the artificial diffusion generated in the mass transfer convection term across the interface is inevitable, especially when large shape deformation is encountered at high Reynolds numbers. A semi-Lagrangian advection scheme is introduced to overcome this disadvantage. The methyl isobutyl ketone (MIBK)-acetic acid-water system is adopted to study the unsteady mass transport process accompanied with the Marangoni effect of a single deformable drop ascending in the infinite continuous phase. The predicted overall mass transfer coefficients agree with experimental data very well. The configuration of Marangoni convection is revealed and its effect on the interphase mass transfer process is investigated.
“…7 a and 7 b. The simulated results reported by Wang et al [33] overestimated significantly compared with the experimental ones, as listed in Tab. 3.…”
Section: Mass Transfer Coefficientscontrasting
confidence: 49%
“…(7). The involved coefficients [33] were given as a = -0.475 and b = 0.06 for Case 1, and a = -0.74 and b = 0.14 for Case 2. …”
The level set method is combined with the concentration transformation method to solve the interphase mass transfer process. However, the artificial diffusion generated in the mass transfer convection term across the interface is inevitable, especially when large shape deformation is encountered at high Reynolds numbers. A semi-Lagrangian advection scheme is introduced to overcome this disadvantage. The methyl isobutyl ketone (MIBK)-acetic acid-water system is adopted to study the unsteady mass transport process accompanied with the Marangoni effect of a single deformable drop ascending in the infinite continuous phase. The predicted overall mass transfer coefficients agree with experimental data very well. The configuration of Marangoni convection is revealed and its effect on the interphase mass transfer process is investigated.
“…Even if the magnitude of Marangoni convection decreases rapidly with the distance from the interface, it changes the heat and mass transfer rates observed in such systems. This effect, already noted in the early experiments of Sherwood & Wei [1], motivated continuing research on Marangoni flow structures and their relation to mass transfer efficiency [2][3][4][5]. Furthermore, new technologies are developed which use these flow structures to pattern functional surfaces [6,7].…”
“…Marangoni flow has been studied experimentally and through numerical and computational modelling . The simulations in these studies have the advantage of viewing the flow effects in more detail . This behaviour is common in pure liquids, but has been found to be far more complex in multiple component systems .…”
The complex patterns observed from evaporated liquid drops have been examined extensively over the last 20 years. Complete understanding of drop deposition is vital in many medical processes, and one which is essential to the translation of biofluid spectroscopic disease diagnostics. The promising use of spectroscopy in disease diagnosis has been hindered by the complicated patterns left by dried biological fluids which may inhibit the clinical translation of this technology. Coffee-ring formation, cracking and gelation patterns have all been observed in biofluid drops, and with surface homogeneity being a key element to many spectroscopic techniques, experimental issues have been found to arise. A better understanding of the fundamental processes involved in a drying droplet could allow efficient progression in this research field, and ultimately benefit the population with the development of a reliable cancer diagnostic.
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