“…TiO 2 has been extensively selected as a preferred material for environmental remediation owing to its chemical stability, low cost, high durability, nontoxicity, photocorrosion resistance, and excellent biocompatibility. , However, the inherent deficiency of wide band gap (3.2 eV), which indicates that TiO 2 only could be excited by UV light, restricts its photocatalytic efficiency and practical application. On account of less than 5% of UV light in the solar pectrum, tremendous works have been conducted to extend the spectral response range of TiO 2 in the visible region, such as heterojunction, surface sensitization, noble metal deposition, and doping foreign elements . Therein, surface sensitization is the most simple and effective pathway to widen the adsorption spectrum with high energy conversion efficiency, which has been widely used in solar cells, environmental remediation, photosynthesis, water splitting, and so forth. ,, In a typical photocatalytic process for dye-sensitized TiO 2 , fast electron transfer (ET) from the surface-bound chromophores to the conduction band of TiO 2 could be obtained under visible-light irradiation, thus resulting in efficient reduction of oxygen for the formation of reactive oxygen species (ROS), such as superoxide anion radical (O 2 •– ), hydroxyl radical ( • OH), and hydrogen peroxide (H 2 O 2 ).…”