2023
DOI: 10.1126/science.adf1065
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Negative refraction in hyperbolic hetero-bicrystals

Abstract: We visualized negative refraction of phonon polaritons, which occurs at the interface between two natural crystals. The polaritons—hybrids of infrared photons and lattice vibrations—form collimated rays that display negative refraction when passing through a planar interface between the two hyperbolic van der Waals materials: molybdenum oxide (MoO 3 ) and isotopically pure hexagonal boron nitride (h 11 BN). At a special frequency ω 0 , the… Show more

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Cited by 39 publications
(19 citation statements)
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“…The near-field intensity distribution of in-plane hyperbolic focusing affected by the polarization is revealed by modulating the relative angle of the NW to the in-plane polarized light, which is of great significance to guide in-plane modulation efforts. Overall, our work provides new possibilities for deeper investigation of light–matter coupling and guidance modes for low-dimensional nanolens, and polarized wave array-type excitation and focusing provide ideas for molecular sensing, light guidance, energy confinement, ,, etc. It also opens the way for the development of planar photonic applications, such as planar nanoswitches and in-plane heat conduction.…”
Section: Discussionmentioning
confidence: 95%
“…The near-field intensity distribution of in-plane hyperbolic focusing affected by the polarization is revealed by modulating the relative angle of the NW to the in-plane polarized light, which is of great significance to guide in-plane modulation efforts. Overall, our work provides new possibilities for deeper investigation of light–matter coupling and guidance modes for low-dimensional nanolens, and polarized wave array-type excitation and focusing provide ideas for molecular sensing, light guidance, energy confinement, ,, etc. It also opens the way for the development of planar photonic applications, such as planar nanoswitches and in-plane heat conduction.…”
Section: Discussionmentioning
confidence: 95%
“…Recently, effects of interface with one side of heterostructure isotopically purified, are studied. Phenomena like hyperfine isotope effects regulating interlayer electron-phonon coupling in heterostructures 26 and visualizing negative refraction of phonon polaritons 27 are reported. However, in the case of heterogeneous distribution of isotopes, the presence of isotope interfaces in a natural material makes it similar to the “superlattice” case.…”
Section: Introductionmentioning
confidence: 98%
“…Infrared near-field nanospectroscopy combines the nanometer spatial resolution of atomic force microscopy with the high information density of optical spectroscopy. Due to its unique capabilities, the technique has continuously been expanding and has been applied to material characterization throughout various fields of engineering, chemistry, geology, and physics. A major and rapidly growing subfield of near-field nanospectroscopy includes polariton interferometry, which provides direct access to the dispersion of deeply subwavelength-confined polariton modes. …”
Section: Introductionmentioning
confidence: 99%