“…10,11 In the past few decades, the efforts to realize high performance LSPR sensors have sparked a plethora of designs such as single metallic nanoparticles, [12][13][14] coupled multimers, 15,16 and periodic nanostructures, [17][18][19][20] and witnessed detection success in many fields including chemistry, 7 biology, 21 medicine, 8 the environment 22 and food safety. 23 To evaluate the sensing performance of LSPRs, it is common to use two characteristics, namely the sensitivity denoted as the peak shift per refractive index unit S = dλ/dn and the figure of merit obtained through dividing the sensitivity by the resonance linewidth, FOM = S/Δλ. Naturally, it is indispensable to greatly increase the sensitivity, but meanwhile reduce the plasmon resonance linewidth to realize an ideal LSPR sensor.…”