We report the direct observation of coupling between a single self-assembled InAs quantum dot and a wetting layer, based on strong diamagnetic shifts of many-body exciton states using magneto-photoluminescence spectroscopy. An extremely large positive diamagnetic coefficient is observed when an electron in the wetting layer combines with a hole in the quantum dot; the coefficient is nearly one order of magnitude larger than that of the exciton states confined in the quantum dots. Recombination of electrons with holes in a quantum dot of the coupled system leads to an unusual negative diamagnetic effect, which is five times stronger than that in a pure quantum dot system. This effect can be attributed to the expansion of the wavefunction of remaining electrons in the wetting layer or the spread of electrons in the excited states of the quantum dot to the wetting layer after recombination. In this case, the wavefunction extent of the final states in the quantum dot plane is much larger than that of the initial states because of the absence of holes in the quantum dot to attract electrons. The
properties of emitted photons that depend on the large electron wavefunction extents in the wetting layer indicate that the coupling occurs between systems of different dimensionality,which is also verified from the results obtained by applying a magnetic field in different configurations. This study paves a new way to observe hybrid states with zero-and two-Nano Res. dimensional structures, which could be useful for investigating the Kondo physics and implementing spin-based solid-state quantum information processing.Semiconductor quantum dots (QDs), also known as "artificial atoms", have attracted considerable interest because of their application to quantum optoelectronic devices such as singlephoton sources [1-6], quantum bits [7,8], quantum logic gates [9], and photon-spin interfaces [10][11][12]. Owing to the quasi-zero-dimensional nature of QDs, many-body effect induced exciton states have been achieved in single QDs by controlling charge states with external electric and magnetic fields [13][14][15]. Following the discovery of graphene [16], two-dimensional materials, such as MoS2 [17, 18] and black phosphorous [19], have been investigated extensively. Recently, the coupling between QDs and two-dimensional extended states has been investigated to demonstrate the Kondo physics [15,[20][21][22][23][24] and Fano effect [25,26]. Hybridization between a single QD and a twodimensional continuum state has been studied experimentally and theoretically in various systems [21,[27][28][29][30][31][32]. For self-assembled QDs grown by molecular beam epitaxy (known as Stranski-Krastanov growth), a wetting layer with a thickness of a few monolayers is always formed underneath the QDs [33][34][35], which naturally provides a platform for the formation of coupled systems for many-body exciton states [15,27]. Karrai et al. [27] have shown the coherent hybridization of localized QD states and extended continuum states in the wetting la...