“…These smart actuators covert the external energy into mechanical energy to implement the predetermined motions under diverse forms of external stimuli, such as DOI: 10.1002/adfm.202311398 electricity, [1,2] humidity, [3][4][5] light, [6][7][8] heat, [9] and magnetics, [10] and they have revealed intriguing and noteworthy applications in artificial tissues, [11] sensors, [12] soft robots, [13][14][15] drug delivery, [16] and energy storage and conversion, [17][18][19] etc. Currently, the inherent characteristics of actuating materials including the photothermal effect of carbon-based materials, [20] the hygroscopicity of hydrogel materials, [21] or contraction of layer interior space in 2D materials, [6,22,23] have been promoted and integrated to evolve the controllable intelligent film actuators with high performance. The patterning of film actuators can be straightforwardly accomplished through various processing techniques including regional vacuum filtration, [24] molding, [25] mask spray coating, photolithography, [26] and direct printing.…”