“…Aggregation is pronounced in highly polar solvents like water and alcohol and restricts the use of these media, although they form ideal components for liquid dye lasers due to their high specific heat and constancy of thermo-optical properties (Tuccio and Strome, 1972). Xanthene dyes, of which Rhodamines form an important group (Peterson et af., 1970;Snarley and Schafer, 1969), have been in very active use as laser dyes.Rhodamines as a class of laser dyes are known for their high water solubilities, but this beneficial property has been marred by the detrimental formation of dimeric aggregates which impair the laser action (Marling et al, 1974). Different approaches adopted to circumvent the dimerization phenomenon include the use of solvents like hexafluoroisopropanol and N,N-dipropylacetamide (Tuccio et al, 1973), and the addition of surfactants as deaggregating agents (Tuccio and Strome, 1972;Marling et al, 1974;Alfano et al, 1973).…”