“…Using these characteristics, 222 Rn is often used as a target tracer to investigate the hydrological aspects of groundwater (e.g., estimation of infiltration from surface water to aquifers [34] and groundwater flow rate [35]), because far more 222 Rn is contained in groundwater than in surface water. The radioactivity of 222 Rn in samples was analyzed using a liquid scintillation counter (Packard, 2250 CA, CT, USA) after extraction with toluene within one week after collecting the water, and the concentrations of 222 Rn were calculated based on the count rate [36]. The stable isotopic compositions of the water were measured using a cavity ringdown spectrometer-based water isotope analyzer (Picarro, L2140-i, Santa Clara, CA, USA).…”