An effective scheme to extend the harmonic cutoff and enhance the harmonic yield from ion by using nano-plasmonic-pump-probe technology has been proposed. The essence of the present scheme is to use the pump pulse to steer to the multi-photon-resonance-ionization region, where the ionization probability can be remarkably enhanced. Then, a sequential probe pulse with a proper delay time can enhance the harmonic yield. Furthermore, by properly choosing the injected position of and by properly adding a controlling pulse, a single harmonic emission event with a broader harmonic plateau can be obtained. Finally, by the Fourier transformation of the selected harmonics on the harmonic plateau, a single 38 as pulse with intensity enhancement of 400 times can be obtained.