2018
DOI: 10.1364/ome.8.003688
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Interference in edge-scattering from monocrystalline gold flakes [Invited]

Abstract: We observe strongly dissimilar scattering from two types of edges in hexagonal quasimonocrystalline gold flakes with thicknesses around 1 micron. We identify as the origin the interference between a direct, quasi-specular scattering and an indirect scattering process involving an intermediate surface-plasmon state. The dissimilarity between the two types of edges is a direct consequence of the three-fold symmetry around the [111]-axis and the intrinsic chirality of a face-centered cubic lattice. We propose tha… Show more

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Cited by 22 publications
(26 citation statements)
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References 30 publications
(36 reference statements)
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“…The NPL is mostly emitted at the edges and apices of the quasi-2D structure [16]. Similar to the gold stripe, the origin of this strong response located at the boundaries is the combining results of the enhancement of the electromagnetic field at the dielectric discontinuity and the particularity of the electronic band structure around the specific atomic orientation of the edges and apices [38].…”
Section: Plasmonic Objectsmentioning
confidence: 97%
“…The NPL is mostly emitted at the edges and apices of the quasi-2D structure [16]. Similar to the gold stripe, the origin of this strong response located at the boundaries is the combining results of the enhancement of the electromagnetic field at the dielectric discontinuity and the particularity of the electronic band structure around the specific atomic orientation of the edges and apices [38].…”
Section: Plasmonic Objectsmentioning
confidence: 97%
“…In the experiment, colloidal gold crystals were grown on a silicon substrate using a thermolysis synthesis technique 38 (see details in Supplementary, Section 2). Lithographic alignment markers were made on top of (and nearby) the gold crystals, and NDs were deposited on the substrate afterwards.…”
Section: Resultsmentioning
confidence: 99%
“…Gold flakes were made following the recipe from ref. [78]. Alignment markers were made on the gold crystals, and subsequently NDs were deposited on the substrate following the process described in Section 3.2.…”
Section: Bragg Cavities and Mirrors For Efficient Channeling Of Emission Into Plasmonic Waveguidesmentioning
confidence: 99%