We report on the controlled coupling of a single nitrogen-vacancy (NV) center to a surface plasmon mode propagating along a chemically grown silver nanowire (NW). We locate and optically characterize a single NV center in a uniform dielectric environment before we controllably position this emitter in the close proximity of the NW. We are thus able to control the coupling of this particular emitter to the NW and directly compare the photon emission properties before and after the coupling. The excitation of single plasmonic modes is witnessed and a total rate enhancement by a factor of up to 4.6 is demonstrated.
Nanofabrication of photonic components based on dielectric-loaded surface plasmon-polariton waveguides (DLSPPWs) excited by single nitrogen vacancy (NV) centers in nanodiamonds is demonstrated. DLSPPW circuits are built around NV containing nanodiamonds, which are certified to be single-photon emitters, using electron-beam lithography of hydrogen silsesquioxane (HSQ) resist on silver-coated silicon substrates. A propagation length of ~20 {\mu}m for the NV single-photon emission is measured with DLSPPWs. A 5-fold enhancement in the total decay rate and up to 63% coupling efficiency to the DLSPPW mode is achieved, indicating significant mode confinement. Finally, we demonstrate routing of single plasmons with DLSPPW-based directional cou-plers, revealing the potential of our approach for on-chip realization of quantum-optical networks
Single photons carrying spin angular momentum (SAM), i.e., circularly polarized single photons generated typically by subjecting a quantum emitter (QE) to a strong magnetic field at low temperatures, are at the core of chiral quantum optics enabling nonreciprocal single-photon configurations and deterministic spin-photon interfaces. Here, a conceptually new approach to the room-temperature generation of SAM-coded single photons (SSPs) is described, which entails QE nonradiative coupling to surface plasmons being transformed, by interacting with an optical metasurface, into a collimated stream of SSPs with the designed handedness. Design, fabrication, and characterization of SSP sources, consisting of dielectric circular nanoridges with azimuthally varying widths deterministically fabricated on a dielectricprotected silver film around a nanodiamond containing a nitrogen-vacancy center, are reported. With properly engineered phases of QE-originated fields scattered by nanoridges, the outcoupled photons are characterized by a well-defined SAM (with the chirality >0.8) and high directionality (collection efficiency up to 92%).Single-photon sources constitute one of the crucial enabling technologies for quantum communications, [1][2][3] quantum computation, [4][5][6] and quantum-enhanced metrology. [7][8][9] Typical stand-alone quantum emitters (QEs) used for realizing singlephoton sources feature low emission rates, nondirectional emission, and poorly defined polarization properties, [10][11][12][13] characteristics that prevent QEs from being directly used in
We report on coupling of a single nitrogen-vacancy (NV) center in a nanodiamond to the propagating gap mode of two parallel placed chemically grown silver nanowires. The coupled NV-center nanowire system is made by manipulating nanodiamonds and nanowires with the tip of an atomic force microscope cantilever. An efficient coupling of an NV-center to an easily accessible gap plasmon mode is demonstrated and we measure an enhancement of the spontaneous emission decay rate by a factor of 8.3.
Monolithic integration of quantum emitters in nanoscale plasmonic circuitry requires low-loss plasmonic configurations capable of confining light well below the diffraction limit. We demonstrated on-chip remote excitation of nanodiamond-embedded single quantum emitters by plasmonic modes of dielectric ridges atop colloidal silver crystals. The nanodiamonds were produced to incorporate single germanium-vacancy (GeV) centres, providing bright, spectrally narrow and stable single-photon sources suitable for highly integrated circuits. Using electron-beam lithography with hydrogen silsesquioxane (HSQ) resist, dielectric-loaded surface plasmon polariton waveguides (DLSPPWs) were fabricated on single crystalline silver plates to contain those of deposited nanodiamonds that are found to feature appropriate single GeV centres. The low-loss plasmonic configuration enabled the 532-nm pump laser light to propagate on-chip in the DLSPPW and reach to an embedded nanodiamond where a single GeV centre was incorporated. The remote GeV emitter was thereby excited and coupled to spatially confined DLSPPW modes with an outstanding figure-of-merit of 180 due to a ~six-fold Purcell enhancement, ~56% coupling efficiency and ~33 μm transmission length, thereby opening new avenues for the implementation of nanoscale functional quantum devices.
We demonstrate an exceptionally bright photon source based on a single nitrogenvacancy center (NV-center) in a nanodiamond (ND), placed in the nanoscale gap between two monocrystalline silver cubes in a dimer configuration. The system is operated near saturation at a stable photon rate of 850 kcps, while we further achieve strongly polarized emission and high single photon purity, evident by the measured auto-correlation with a g (2) (0)-value of 0.08. These photon source features are key parameters for quantum technological applications, such as secure communication based on quantum key distribution. The cube antenna is assembled with an atomic force microscope, which allows us to predetermine the dipole orientation of the NV-center and optimize cube positioning accordingly, while also tracking the evolution of emission parameters from isolated ND to the 1 and 2 cube configuration. The experiment is well described by finite element modelling, assuming an instrinsic quantum efficiency of 0.35. We attribute the large photon rate of the assembled photon source, to increased quantum efficiency of the NV-center and high antenna efficiency.
A room-temperature on-chip orbital angular momentum source that emits well-collimated single photons has been demonstrated.
Quantum emitters with high emission rates and efficiently coupled to optical waveguides are in demand for various applications in quantum information technologies. Accurate positioning of a quantum emitter within a strongly confined gap-plasmon waveguide (GPW) mode would allow one to significantly enhance the decay rate and efficiency of channeling of emitted photons into the waveguide mode. Here, we present experimental results on the GPW mode excitation in a gap between a monocrystalline silver nanowire and a monocrystalline silver flake by using a single nitrogen-vacancy center in a nanodiamond. The coupled systems containing a nanodiamond and the structure supporting the GPW mode are created by a combination of electron beam lithography and nano manipulation with an atomic force microscope (AFM). In these systems, we find the decay rate enhancements of up to~50, and the efficiency of channeling of photons into the GPW mode of up to 82%, resulting in an exceptionally high figure-of-merit of 212 for the emitter-plasmonic waveguide coupled system. The 1 results obtained suggest new avenues for practical realization of integrated solid-state quantum systems.
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