A novel combination of low-field magnetic alignment (MA) and templated grain growth (TGG) was used to fabricate highly textured diamagnetic 0.72Pb(Mg 1/3 Nb 2/3 )O 3 -0.28PbTiO 3 (0.72PMN-0.28PT) ceramics. Samples were produced by nonaqueous slip casting of PMN-PT slurries, in which diamagnetic plate-like 0.4(Na 1/2 Bi 1/2 )TiO 3 -0.6PbTiO 3 (0.4NBT-0.6PT) template particles were aligned by dynamic MA in a 2.2-T permanent magnet array. Template alignment improved as slurry viscosity increased, with a 32-vol% solid loading (a viscosity of ;0.1 Pa s at 0.1 s À1 ) giving optimal texture quality (7.85°FWHM, f 5 92 vol%) after sintering and TGG. Alignment was stable for more than 3 h during slip casting, allowing fabrication of ;1-cm thick textured ceramics with high piezoelectric response (d 33 5 1222 pC/N). The success of dynamic MA at low magnetic field (2.2 T) is attributed to an increase in driving force for alignment of large (5-10 lm) template particles relative to the randomizing effect of Brownian motion (i.e., thermal energy k B T).