Precious organic cultural relics are easily affected by temperature, humidity, and harmful gases in the environment, resulting in embrittlement, fading, mildew, moth damage and other aging forms. An energy-saving and environmentally friendly material is needed to stabilize humidity and adsorb harmful gases in the environment. In this paper, with an intelligent adjustment function, functional paper containing sepiolite and tourmaline natural minerals was successfully prepared. The component of 80 % of wingceltis and 20 % of straw in dry pulp as main raw material was conducive to the desorption of water molecules. As favorable structure inside functional paper, the adsorption point and the adsorption contact area increased by the rough surface of fiber bundles, the addition of sepiolite and the ordered molecular chains of copolymers destroyed. So, the relative humidity could be adjusted to 55 % ± 3 within 2 hours and was stable with functional paper. At the same time, 1.11 ppm sulfur dioxide and 2.98 ppm ammonia could be effectively adsorbed in 10 and 12 h, respectively, by 1 g of paper in a 5 L container. The pH of the paper was adjusted to neutral with tourmaline, even if the pH was changed by acidic or alkaline gas absorption. Therefore, for long-term organic cultural relic preservation, preparing a constant-humidity and clean environment is of great significance. This is possible through this paper.