a b s t r a c tA theoretical model has been developed to illustrate the effect of shear-coupled migration of grain boundaries on dislocation emission in nanocrystalline materials. The energy characteristics and critical shear stress τ c that is required to initiate the emission process were determined. The results obtained show that the dislocation emission can be considerably enhanced as shear-coupled migration was the dominating process; a critical coupling factor that corresponded to the minimum τ c , which led to an optimal dislocation emission, was also discovered. The proposed model has also been quantitatively validated by the existing molecular dynamics simulations.