This paper evaluates the performance of a bimodal carbon fiber cathode and a carbon-epoxy multicapillary cathode operating within a reflex-triode sealed-tube virtual cathode oscillator (vircator). The experimental results reveal that both cathodes exhibit similar emission behavior, although with some significant operational differences. An eight-stage 84-J pulseforming network-based Marx generator serves to drive both cathodes at 250 kV and 3-4 kA with a ∼70-ns pulsewidth. Both cathodes undergo conditioning over 10 000 pulses to determine gas evolution as well as electrical changes over time. Gas evolution of both cathodes is observed using a residual gas analyzer to determine individual gas constituents. A comparison of diode voltage, diode current, RF output, and outgassing data for both cathodes during vircator operation over 10 000 pulses is presented to quantify cathode performance in a sealed-tube vircator. Changes in cathode surface morphology, from virgin to postmortem, are discussed. Data for various anode-cathode gap distances, from 3 to 15 mm, are presented. The evolution of voltage and current inputs to the vircator is discussed.