One
goal of the second quantum revolution is developing an approach
to transmit coherent quantum information across the
world, forming the basis of the quantum Internet. Achieving this lofty
goal will require scalable and tunable materials that allow for cross-platform
interconnections. Solution-processable molecular systems designed
from the ground up are poised to introduce the necessary tunability
to meet these needs. In this Perspective, we describe the components
of a quantum network, outline the criteria to create molecular systems
suitable for networking applications, and discuss the pathway to generate
spin-photon entanglement, a first step toward remote entanglement
between molecular spins in a network. We also describe some initial
steps to optimize molecular spins for potential integration into quantum
networks as readily deployable qubits in network nodes. Throughout
this Perspective, we highlight the tremendous potential of molecular
systems for the quantum Internet and illustrate openings for chemists
in this nascent field.