Identification and optimization of advanced phosphors using combinatorial libraries

Sun, Xiaodong; Chen, Gao; Wang, Jingsong; Xiang, X.‐D.

doi:10.1063/1.119168

Cited by 92 publications

(34 citation statements)

References 8 publications

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“…Sun et al 179 were the first to show the utility of the combinatorial approach for luminescent materials. Using precursor layers deposited by RF sputtering through a set of physical masks, they fabricated thin film libraries to investigate RE activated refractory metal oxides, Gd(La,Sr)AlO x .…”

Section: -23mentioning

confidence: 99%

Applications of high throughput (combinatorial) methodologies to electronic, magnetic, optical, and energy-related materials

Green

Takeuchi

Hattrick‐Simpers

2013

Journal of Applied Physics

223

189

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High throughput (combinatorial) materials science methodology is a relatively new research paradigm that offers the promise of rapid and efficient materials screening, optimization, and discovery. The paradigm started in the pharmaceutical industry but was rapidly adopted to accelerate materials research in a wide variety of areas. High throughput experiments are characterized by synthesis of a "library" sample that contains the materials variation of interest (typically composition), and rapid and localized measurement schemes that result in massive data sets. Because the data are collected at the same time on the same "library" sample, they can be highly uniform with respect to fixed processing parameters. This article critically reviews the literature pertaining to applications of combinatorial materials science for electronic, magnetic, optical, and energy-related materials. It is expected that high throughput methodologies will facilitate commercialization of novel materials for these critically important applications. Despite the overwhelming evidence presented in this paper that high throughput studies can effectively inform commercial practice, in our perception, it remains an underutilized research and development tool. Part of this perception may be due to the inaccessibility of proprietary industrial research and development practices, but clearly the initial cost and availability of high throughput laboratory equipment plays a role. Combinatorial materials science has traditionally been focused on materials discovery, screening, and optimization to combat the extremely high cost and long development times for new materials and their introduction into commerce. Going forward, combinatorial materials science will also be driven by other needs such as materials substitution and experimental verification of materials properties predicted by modeling and simulation, which have recently received much attention with the advent of the Materials Genome Initiative. Thus, the challenge for combinatorial methodology will be the effective coupling of synthesis, characterization and theory, and the ability to rapidly manage large amounts of data in a variety of formats. V C 2013 AIP Publishing LLC. [http://dx

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Section: -23mentioning

confidence: 99%

Applications of high throughput (combinatorial) methodologies to electronic, magnetic, optical, and energy-related materials

Green

Takeuchi

Hattrick‐Simpers

2013

Journal of Applied Physics

223

189

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“…Such measurements include the photoluminescence of phosphors, 4 the spectral reflectance to quantify the color of decorative films, 5 and the thin film a) Authors to whom correspondence should be addressed. Electronic addresses: mitrovic@caltech.edu and gregoire@caltech.edu optical interference pattern to measure film thickness and etch rate.…”

Section: Introductionmentioning

confidence: 99%

High-throughput on-the-fly scanning ultraviolet-visible dual-sphere spectrometer

Mitrović

Cornell

Marcin

et al. 2015

Review of Scientific Instruments

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A new simple and low cost scattered transmission accessory for commercial double beam ultraviolet-visible spectrophotometers Rev. Sci. Instrum. 68, 4288 (1997); 10.1063/1.1148344 This article is copyrighted as indicated in the article. Reuse of AIP content is subject to the terms at: http://scitationnew. We have developed an on-the-fly scanning spectrometer operating in the UV-visible and near-infrared that can simultaneously perform transmission and total reflectance measurements at the rate better than 1 sample per second. High throughput optical characterization is important for screening functional materials for a variety of new applications. We demonstrate the utility of the instrument for screening new light absorber materials by measuring the spectral absorbance, which is subsequently used for deriving band gap information through Tauc plot analysis. C 2015 AIP Publishing LLC. [http://dx

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“…SCHULTZ, XIANG, and coworkers [155][156][157][158] used thin-film deposition methods and physical masking-techniques to synthesize spatially defined libraries of solid-state thin films. The individual element precursors of interest were sequentially sputtered onto the surface of a single-crystal wafer of magnesium oxide or lanthanum aluminate through a series of physical masks.…”

Section: Combinatorial Chemistry and Materials Sciencementioning

confidence: 99%

Combinatorial Chemistry

Tiebes

Peters

2000

Ullmann's Encyclopedia of Industrial Chemistry

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The article contains sections titled: 1. Introduction 2. Concept of Combinatorial Chemistry 3. Methods and Techniques of Combinatorial Synthesis 3.1. Synthetic Strategies Towards Combinatorial Libraries 3.1.1. Split ‐ Pool Synthesis Towards Combinatorial Libraries 3.1.1.1. Techniques using Resin Beads 3.1.1.2. Tea‐Bag Method 3.1.2. Parallel Synthesis Towards Combinatorial Libraries 3.1.2.1. Reaction Apparatus using Resin Beads 3.1.2.2. Multipin Technique 3.1.2.3. Spatially Addressable Parallel Synthesis on Silica Wafer 3.1.3. Reagent Mixture Synthesis Towards Combinatorial Libraries 3.2. Synthetic Methodology for Organic Library Construction 3.2.1. Solid‐Phase Organic Synthesis 3.2.1.1. Solid Support, Linker, and Cleavage Strategies 3.2.1.2. Reaction Portfolio 3.2.2. Synthesis in Solution and Liquid‐Phase Synthesis 4. Characterization of Combinatorial Libraries 4.1. Analytical Characterization 4.2. Hit Identification in Combinatorial Libraries by High‐Throughput Screening 4.2.1. Strategies for Libraries of Compound Mixtures 4.2.1.1. On‐Bead Screening 4.2.1.2. Deconvolution 4.2.1.2.1. Iterative Deconvolution 4.2.1.2.2. Deconvolution by Positional Scanning 4.2.1.2.3. Deconvolution by Orthogonal Libraries 4.2.1.3. Encoding 4.2.1.4. Multiple Cleavable Linkers 4.2.2. Strategies for Libraries of Separate Single Compounds 4.2.3. Conclusion 5. Automation and Data Processing 5.1. Synthesis Automation and Data Processing 5.2. Automated Purification 6. Library Design and Diversity Assessment 6.1. Diversity Assessment for Selection of Building Blocks or Compound 6.2. Iterative Optimization Methods 7. Economic Aspects and Industrial Case Studies 8. Further Developments 8.1. Combinatorial Chemistry and Catalysis 8.2. Combinatorial Chemistry and Material Science

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Identification and optimization of advanced phosphors using combinatorial libraries

Cited by 92 publications

References 8 publications

Applications of high throughput (combinatorial) methodologies to electronic, magnetic, optical, and energy-related materials

Applications of high throughput (combinatorial) methodologies to electronic, magnetic, optical, and energy-related materials

High-throughput on-the-fly scanning ultraviolet-visible dual-sphere spectrometer

Combinatorial Chemistry

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