2006
DOI: 10.1103/physrevlett.96.153001
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High Resolution Atomic Coherent Control via Spectral Phase Manipulation of an Optical Frequency Comb

Abstract: We demonstrate high resolution coherent control of cold atomic rubidium utilizing spectral phase manipulation of a femtosecond optical frequency comb. Transient coherent accumulation is directly manifested by the enhancement of signal amplitude and spectral resolution via the pulse number. The combination of frequency comb technology and spectral phase manipulation enables coherent control techniques to enter a new regime with natural linewidth resolution.

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Cited by 74 publications
(47 citation statements)
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“…To account for the frequency doubling process, the 389 nm light field strength is reduced to 5 × 10 6 V/m and the transform limited pulse length is increased to 65 fs, reflecting spectral narrowing due to phase matching limitations. Although for these simulations the spectral phase is assumed flat, the effect of pulse chirp is small in the case of multipulse excitation of a two-photon transition with a resonant intermediate state [26].…”
Section: Numerical Simulation Of Near-resonant Dfcs Transitions To N mentioning
confidence: 99%
See 1 more Smart Citation
“…To account for the frequency doubling process, the 389 nm light field strength is reduced to 5 × 10 6 V/m and the transform limited pulse length is increased to 65 fs, reflecting spectral narrowing due to phase matching limitations. Although for these simulations the spectral phase is assumed flat, the effect of pulse chirp is small in the case of multipulse excitation of a two-photon transition with a resonant intermediate state [26].…”
Section: Numerical Simulation Of Near-resonant Dfcs Transitions To N mentioning
confidence: 99%
“…The self-calibrating capability of the comb permits accurate determination of atomic structure in alkali and alkaline earth atoms [19,20,21,22,23,24], as well as the investigation of multiple molecular transitions [25]. Furthermore, high-resolution quantum control can be achieved via spectral manipulation of frequency combs [26,27].…”
Section: Introductionmentioning
confidence: 99%
“…DOI: 10.1103/PhysRevLett.104.140501 PACS numbers: 03.67.Bg, 32.80.Qk, 37.10.Rs, 37.10.Vz The optical frequency comb generated from an ultrafast laser pulse train has revolutionized optical frequency metrology [1][2][3][4] and is now playing an important role in high resolution spectroscopy [5]. The spectral purity yet large bandwidth of optical frequency combs also provides a means for the precise control of generic quantum systems, with examples such as the quantum control of multilevel atomic systems [6,7], laser cooling of molecules or exotic atomic species [8,9], and quantum state engineering of spins in semiconductors [10,11] or rovibrational states in molecules [12,13]. The optical frequency comb may become a crucial component in the field of quantum information science, where complex multilevel quantum systems must be controlled with great precision [14].…”
mentioning
confidence: 99%
“…By using a comb laser, which means an ultrafast laser pulse train with a high repetition rate, one can carry out the ultrahigh resolution spectroscopy. Recently it has been shown that the accumulation ef-fects of coherence by a laser pulse train play an important role for coherent control of atomic or molecular systems [9,10]. The use of a chirped laser pulse train is another way for coherent control of population transfer [11].…”
Section: Introductionmentioning
confidence: 99%