We theoretically investigate above-threshold ionization of Mg by linearly and circularly polarized fs laser pulses. We find that the above-threshold ionization peaks are accompanied by small subpeaks for both linearly and circularly polarized pulses. We interpret the physical origin of the subpeaks as above-threshold ionization from the low-lying bound states which are far off-resonantly excited by the spectral wing of the pulse. This interpretation is confirmed by our comparative numerical studies. Furthermore, we provide a clear explanation of why this kind of subpeak in the photoelectron energy spectra has not been reported for smaller photon energies with Mg and other commonly used atoms such as H and rare gas atoms.In order to study the interaction of Mg, a two-valenceelectron system, with a fs laser pulse, we solve the TDSE on *
We theoretically investigate how the photoelectron angular distribution is altered by the introduction of a dressing laser. The physical mechanism underlying this alteration is the so-called laser-induced continuum structure; namely, a strong dressing laser induces quantum mechanical interference, the degree of which is different for different ionization channels. Therefore the branching ratio into different ionization channels changes as a function of laser detuning, and accordingly the photoelectron angular distribution is altered. After a general argument, we present specific theoretical results for the K atom, which indeed exhibit significant modification of the photoelectron angular distribution.
The inelastic scattering of fast electrons by metastable hydrogen atoms in the presence of a linearly polarized laser field is theoretically studied in the domain of field intensities below 10 10 W/cm 2 . The interaction of the hydrogen atom with the laser field is described by first-order time-dependent perturbation theory, while the projectile electrons interacting with the laser field are described by the Gordon-Volkov wave functions. An analytic expression is obtained for the differential scattering cross section in the first-order Born approximation for laser-assisted inelastic e − -H(2s) scattering for the 2s → nl excitation. Detailed analytical and numerical results are presented for inelastic scattering accompanied by one-photon absorption, and the angular dependence and resonance structure of the differential cross sections is discussed for the 2s → 4l excitation of metastable hydrogen.
We theoretically study multiphoton ionization of Mg in the circularly as well as the linearly polarized laser fields. Specifically two-, three-, and four-photon ionization cross sections from the ground and first excited states are calculated as a function of photon energy. Calculations are performed using the frozen-core Hartree-Fock and also the model potential approaches and the results are compared. We find that the model potential approach provide results as good as or even slightly better than those by the frozen-core Hartree-Fock approach. We also report the relative ratios of the ionization cross sections by the circularly and linearly polarized laser fields as a function of photon energy, which exhibit clear effects of electron correlations.
We investigate the dynamics of a pair of short laser pulse trains propagating in a medium consisting of three-level Λ-type atoms by numerically solving the Maxwell-Schrödinger equations for atoms and fields. By performing propagation calculations with different parameters, under conditions of electromagnetically induced transparency, we compare the propagation dynamics by a single pair of probe and coupling laser pulses and by probe and coupling laser pulse trains. We discuss the influence of the coupling pulse area, number of pulses, and detunings on the probe laser propagation and realization of electromagnetically induced transparency conditions, as well on the formation of a dark state.
We theoretically study multiphoton ionization through the triplet states of Mg by linearly polarized and circularly polarized fs laser pulses. After the construction of the atomic basis using the frozen-core Hartree-Fock potential as well as the model potential approaches for both singlet and triplet series which show rather good agreements with the existing data in terms of state energies and dipole matrix elements, we solve time-dependent Schrödinger equations with 3s3p 3 P 1 as an initial state, and calculate the total ionization yield and photoelectron energy spectra.
In this paper we report the theoretical results obtained for partial ionization yields and the above-threshold ionization (ATI) spectra of Magnesium in a Ti:sapphire laser field (804 nm) in the range of short pulse duration (20-120 fs). Ionization yield, with linearly polarized light for a 120 fs laser pulse, is obtained as a function of the peak intensity motivated by recent experimental data [9]. For this, we have solved the time-dependent Schrödinger equation nonperturbatively on a basis of discretized states obtained with two different methods; one with the two-electron wavefunction relaxed at the boundaries, giving a quadratic discretized basis and the other with the two-electron wavefunction expanded in terms of Mg + -orbitals plus one free electron allowing the handling of multiple continua (open channels). Results, obtained with the two methods, are compared and advantages and disadvantages of the open-channel method are discussed.PACS. 3 2.80.Rm Multiphoton ionization and excitation to highly excited states (e.g., Rydberg states)
We theoretically investigate the effects of laser polarization on photoelectron angular distribution through laser-induced continuum structure. We focus on a polarization geometry where the probe and dressing lasers are both linearly polarized, and change the relative polarization angle between them. We find that the total ionization yield and the branching ratio into different ionization channels change as a function of the relative polarization angle, and accordingly the photoelectron angular distribution is altered. We present specific results for the 4p 1/2 -6p 1/2 and 4p 3/2 -6p 3/2 systems of the K atom, and show that the change of the polarization angle leads to the significant modification of photoelectron angular distribution.
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