“…Terbium-aluminum garnet, Tb 3 A l5 O 12 (TAG), has been reported to show the best paramagnetic magneto-optical properties in the visiblenear IR spectral region with a high light transmission coefficient and a high Verdet constant [10], nevertheless, its incongruent melting nature and unstable TAG phase in the Tb 2 O 3 -Al 2 O 3 system have so far impeded the growth of industrially practicable crystals [11]. With the lack of TAG, terbium-gallium garnet, Tb 3 Ga 5 O 12 (TGG) crystal, the next-best magneto-optical material of TAG [12], was introduced as Faraday isolators for high-power laser machinery [13], and make up for the deficiency of YIG in the visible and near infrared spectral regions.…”