2016
DOI: 10.1002/adma.201600160
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Giant Resistive Switching via Control of Ferroelectric Charged Domain Walls

Abstract: Controlled switching of resistivity in ferroelectric thin films is demonstrated by writing and erasing stable, nanoscale, strongly charged domain walls using an in situ transmission electron microscopy technique. The resistance can be read nondestructively and presents the largest off/on ratio (≈10(5) ) ever reported in room-temperature ferroelectric devices, opening new avenues for engineering ferroelectric thin-film devices.

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Cited by 90 publications
(87 citation statements)
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“…Similarly, resonant tunneling could be at the origin of the oscillations observed in the I-V curve at high voltages in Ref. 59. However, these experimental curves do not show clear NDR and the oscillations are clearly weaker than in our calculations.…”
Section: B Resonant Tunnelingcontrasting
confidence: 48%
“…Similarly, resonant tunneling could be at the origin of the oscillations observed in the I-V curve at high voltages in Ref. 59. However, these experimental curves do not show clear NDR and the oscillations are clearly weaker than in our calculations.…”
Section: B Resonant Tunnelingcontrasting
confidence: 48%
“…Therefore, we argue that, in these particular instances presented in Fig. 4, the DW length is a primary factor, but this may not always be the case, and charged versus uncharged DW fractions might be a predominant factor in other cases ( 27 ). …”
Section: Resultsmentioning
confidence: 88%
“…Besides DW length, relative fractions of charged versus uncharged DW segments are also an important consideration ( 27 ), which can explain the behavior observed in Fig. 4H.…”
Section: Resultsmentioning
confidence: 90%
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“…Finally, synergy of SPM and high resolution STEM can reveal associated mechanisms of the atomic level. 209,379,[404][405][406] Further broad opportunities are opened by implementation of these techniques in liquid environments. 329,[407][408][409][410] While in this case electromechanical responses of material will compete with that of polarizable liquids 411,412 , these studies will provide insight into electromchanical couplings in biological systems and open the window into electro mechanics of molecular systems, the crucial development that will allow not only "to think" but also "to act" on the nanoscale.…”
Section: Discussionmentioning
confidence: 99%