2009
DOI: 10.1103/physrevlett.102.187201
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Giant Modification of the Magnetocrystalline Anisotropy in Transition-Metal Monolayers by an External Electric Field

Abstract: Controlling and designing quantum magnetic properties by an external electric field is a key challenge in modern magnetic physics. Here, from first principles, the effects of an external electric field on the magnetocrystalline anisotropy (MCA) in ferromagnetic transition-metal monolayers are demonstrated which show that the MCA in an Fe(001) monolayer [but not in Co(001) and Ni(001) monolayers] can be controlled by the electric field through a change in band structure, in which small components of the p orbit… Show more

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Cited by 351 publications
(232 citation statements)
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“…This affects the surface MCA owing to the different contribution of these orbitals to the MCA energy [112]. Recent first-principles calculations have demonstrated the importance of these effects [128,129]. Recently, a strong effect of applied electric field on the interface MCA was demonstrated for the Fe/MgO (001) interfaces [130].…”
Section: (B) Surface Magnetocrystalline Anisotropymentioning
confidence: 99%
“…This affects the surface MCA owing to the different contribution of these orbitals to the MCA energy [112]. Recent first-principles calculations have demonstrated the importance of these effects [128,129]. Recently, a strong effect of applied electric field on the interface MCA was demonstrated for the Fe/MgO (001) interfaces [130].…”
Section: (B) Surface Magnetocrystalline Anisotropymentioning
confidence: 99%
“…As the majority of these materials loses their ferromagnetic properties at room temperature the recent discovery of an important ME effect at room temperature in conventional ferromagnetic metals 3-8 has attracted much attention. Despite the limited penetration depth of an E-field in metals, the charge induced at the metal/dielectric interface on the topmost atomic layers is sufficient to modify the surface magnetic anisotropy energy (MAE) by a non negligible amount in ultrathin ferromagnetic layers as suggested by electronic structure calculations [9][10][11] . This has a particular impact in systems where the different anisotropy contributions almost cancel each other out, resulting in a large relative variation of the total effective MAE when the surface contribution is modified with the voltage [12][13][14][15][16][17][18][19][20][21][22][23][24][25][26] .…”
mentioning
confidence: 99%
“…This effect can be induced by purely electronic effects and by chemical or mechanical effects. The physical mechanisms of the purely electronic VCMA effect have been interpreted as the modification of the electronic structure at the interface through charge accumulation/depletion, [21][22][23] an electricfield-induced magnetic dipole 24 or the Rashba effect. 25 Chemical effects, such as a voltage-induced redox reaction, 26 or other electromigration 27 or charge trapping 28 effects can show a substantial VCMA coefficient of the order of a few thousands of fJ Vm − 1 , which is defined as the induced surface anisotropy energy change per unit electric field.…”
Section: Introductionmentioning
confidence: 99%