2015
DOI: 10.1039/c5sm00718f
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Geometric pumping in autophoretic channels

Abstract: Many microfluidic devices use macroscopic pressure differentials to overcome viscous friction and generate flows in microchannels. In this work, we investigate how the chemical and geometric properties of the channel walls can drive a net flow by exploiting the autophoretic slip flows induced along active walls by local concentration gradients of a solute species. We show that chemical patterning of the wall is not required to generate and control a net flux within the channel, rather channel geometry alone is… Show more

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Cited by 34 publications
(43 citation statements)
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“…In this work, we demonstrated the emergence of spontaneous convective flows within a straight phoretic channel whose active walls drive a fluid flow in response to self-induced gradients of a chemical species. This mechanism, which is similar to a Bénard-Marangoni instability, identifies therefore a new route to the emergence of phoretic flows within a chemically-active micro-channel, in addition to asymmetric designs in chemical activity [16] or wall geometry [14], similarly to the dual problem of emergence of self-propulsion for phoretic colloids. A major difference between phoretic particles and channels need to be emphasized.…”
Section: Discussionmentioning
confidence: 90%
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“…In this work, we demonstrated the emergence of spontaneous convective flows within a straight phoretic channel whose active walls drive a fluid flow in response to self-induced gradients of a chemical species. This mechanism, which is similar to a Bénard-Marangoni instability, identifies therefore a new route to the emergence of phoretic flows within a chemically-active micro-channel, in addition to asymmetric designs in chemical activity [16] or wall geometry [14], similarly to the dual problem of emergence of self-propulsion for phoretic colloids. A major difference between phoretic particles and channels need to be emphasized.…”
Section: Discussionmentioning
confidence: 90%
“…We first focus on the linear stability analysis of this system around the steady state from Eq. (14). Decomposing c =c + c and ψ = ψ , the linearized problem for c is obtained as…”
Section: Linear Stability Analysis Of the Steady Statementioning
confidence: 99%
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“…The physico-chemical principles used for phoretic swimmers can in principle also be exploited to induce flow transport in confined devices such as microchannels, and therefore to create pumps [26][27][28][29]. Yet, the existing literature has only so far provided limited insight on the fundamental design principles of such pumps, and we propose here a detailed analysis of the link between pump design and performance.…”
Section: Introductionmentioning
confidence: 99%
“…Moreover, the fact that in-and outlets rely on external pieces of equipment, importantly hampers the portability of the devices. A competitive approach is to induce stresses localized at the boundaries, through non-mechanical means which are driven typically by local fields [12][13][14][15][16]. This has shown to be especially efficient for miniaturizing fluidic pumps, due to the intrinsic large surface to volume ratio.…”
Section: Introductionmentioning
confidence: 99%