2008
DOI: 10.1007/s00340-008-2993-7
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Generation and application of high power femtosecond pulses in the vibrational fingerprint region

Abstract: We present a novel high power femtosecond infrared laser source, based on a three-stage chirped-pulse amplification scheme. Owing to the high power output of the Ti:sapphire amplifiers, it becomes routinely possible to produce femtosecond infrared laser pulses in the wavelength region of 2.6-20 µm with minimum pulse energies of 15 µJ, to our knowledge roughly an improvement of an order of magnitude. With such pulses we have performed femtosecond second-order nonlinear optical surface spectroscopy in the finger… Show more

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Cited by 42 publications
(38 citation statements)
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“…Since at least one of the frequencies involved in a three-wave mixing process is necessarily well separated from the others, second-order processes represent in a natural way an excellent candidate for generating mid-IR and far-IR wavelengths [31]. Efficient nonlinear conversion require materials with strong nonlinearities, high-optical intensities, and phase-matching between the waves involved [13].…”
Section: Difference-frequency Generation (Dfg)mentioning
confidence: 99%
“…Since at least one of the frequencies involved in a three-wave mixing process is necessarily well separated from the others, second-order processes represent in a natural way an excellent candidate for generating mid-IR and far-IR wavelengths [31]. Efficient nonlinear conversion require materials with strong nonlinearities, high-optical intensities, and phase-matching between the waves involved [13].…”
Section: Difference-frequency Generation (Dfg)mentioning
confidence: 99%
“…Assuming further that the nonlinear susceptibility is non-zero only inside the slot, we evaluate numerically the integrals Eq. (5), (6) for the geometry considered in Fig. 3, and find …”
mentioning
confidence: 94%
“…Since at least one of the frequencies involved in a three-wave mixing process is necessarily well separated from the others, second-order processes represent additionally an excellent candidate for generating mid-IR and far-IR wavelengths [6]. Efficient nonlinear conversions require materials with strong nonlinearities, high-optical intensities and phase-matching between the waves involved [1].…”
Section: Introductionmentioning
confidence: 99%
“…Cascaded high-energy OPA-systems have nonetheless been implemented in which a second stage of parametric frequency conversion (mostly DFG) enables reaching the mid-IR spectral range at the expense of efficiency and simplicity [201,202,203]. Maximum pulse energies up to 100 µJ at 4 µm with 1 610 kHz repetition rate [202] could be demonstrated. In contrast, OPCPA enables order of magnitude further upscaling of the output energies.…”
mentioning
confidence: 99%