2022
DOI: 10.1039/d1ta09154a
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Facile fabrication of single-atom catalysts by a plasma-etching strategy for oxygen reduction reaction

Abstract: Single-atom catalysts (SACs) are one of the most promising candidates to catalyze various electrochemical reactions, due to the maximum atom utilizations and unique electronic structures. However, the general methods for...

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Cited by 26 publications
(10 citation statements)
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References 48 publications
(46 reference statements)
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“…In contrast to the previously reported impregnation methods that rely on the physical capture between the metal precursor and the support in the solvent, the efficiency of single-atom vapor deposition depends on the pore structure of the MOF to avoid agglomeration, thus achieving a high load of the metal content. 30,31 X-ray diffraction (XRD) patterns (Fig. 2a) of the Fe-SA/NC catalysts presented two broad peaks for the graphite carbon.…”
Section: Synthesis and Characterizations Of Fe-sa/nc Catalystmentioning
confidence: 99%
“…In contrast to the previously reported impregnation methods that rely on the physical capture between the metal precursor and the support in the solvent, the efficiency of single-atom vapor deposition depends on the pore structure of the MOF to avoid agglomeration, thus achieving a high load of the metal content. 30,31 X-ray diffraction (XRD) patterns (Fig. 2a) of the Fe-SA/NC catalysts presented two broad peaks for the graphite carbon.…”
Section: Synthesis and Characterizations Of Fe-sa/nc Catalystmentioning
confidence: 99%
“…A large number of defects on the NC capture and anchor Cu atoms forming the active site of Cuā€poā€N 3 with a theoretical overpotential of only 0.21 V and excellent stability. [ 74 ]…”
Section: Enhancing the Intrinsic Activity Of The Active Sitesmentioning
confidence: 99%
“…Cu SACs are emerging as promising catalysts and attracting great interest for driving some key reactions, such as electrocatalytic energy conversion (e.g. electrocatalytic CO 2 reduction, [78][79][80][81] oxygen reduction reaction, [82][83][84] nitrogen reduction reaction, 85 and nitrate reduction reaction 86,87 ), photocatalytic reactions (e.g. photocatalytic CO 2 reduction 88 and hydrogen evolution reaction 89,90 ) and heterogeneous reactions (e.g.…”
Section: Non-noble Metal Single-atom Catalystsmentioning
confidence: 99%