It remains a challenge to independently manipulate the magnetic dipolar and the spin-exchange interactions, which are entangled in many spin systems, particularly in spin-1 Bose-Einstein condensates. For this purpose, we put forward a sequence of rf pulses and the periodic dynamical decoupling sequence of optical Feshbach resonance pulses to control the dipolar and the spin-exchange interactions, respectively. Our analytic results and the numerical simulations demonstrate that either of the two interactions can be suppressed to make the other dominate the spin dynamics; furthermore, both of the interactions can be simultaneously suppressed to realize spinor-condensate-based magnetometers with a higher sensitivity. This manipulation method may find its wide applications in magnetic resonance and spintronics. PACS numbers: 03.75.Mn, 03.75.Kk, 03.67.PpIntroduction-Long-range magnetic dipolar interaction and short-range spin-exchange interaction are fundamental in many spin systems, such as the electron and nuclear spin systems [1], the ferromagnetic ultrathin films [2], the ultracold atomic and molecular gases [3,4], and so on. The competition between the two spin interactions diversifies not only the ground state but also the spin dynamics, especially in spinor [5][6][7][8][9][10][11] or dipolar Bose-Einstein condensates (BECs) [12][13][14][15][16][17][18], where the internal spin degrees of freedom are released in optical traps [19,20] and many physical parameters can be tuned precisely. However, the entanglement of the dipolar and spin-exchange interactions makes it difficult to understand the observed phenomena in many experiments. Such an interesting example is the spin texture or the spin domain in 87 Rb spin-1 condensates, which might be ascribed to either one of these two interactions or both of them [21,22]. Accordingly, it is highly desired to suppress one spin interaction and make the other dominant. Although efforts have been made to prohibit either the dipolar interaction [21] or the spin exchange interaction [23,24], it is yet difficult to clearly separate the individual effects.In this paper, we propose to independently suppress the dipolar and the spin-exchange interaction by a sequence of rf pulses ( Fig. 1) and optical Feshbach periodic dynamical decoupling (PDD) sequences [24], respectively. This scheme was verified by the analytic derivations, demonstrating that the manipulations of the relative strength between the two spin interactions enable experimentalists to unambiguously distinguish the specific role of the dipolar and the spin-exchange interactions. It is notable that the sequence of rf pulses is similar to the so called WAHUHA rf pulse sequence