Recently,
multifunctional devices printed on flexible substrates, with multisensing
capability, have found new demand in practical fields of application,
such as wearable electronics, soft robotics, interactive interfaces,
and electronic skin design, revealing the vital importance of precise
control of the fundamental properties of metal oxide nanomaterials.
In this paper, a novel low-cost and scalable processing strategy is
proposed to fabricate all-printed multisensing devices with UV- and
gas-sensing capabilities. This undertaken approach is based on the
hierarchical combination of the screen-printing process and laser
irradiation post-treatment. The screen-printing is used for the patterning
of silver interdigitated electrodes and the active layer based on
anatase TiO2 nanoparticles, whereas the laser processing
is utilized to fine-tune the UV and ethanol-sensing properties of
the active layer. Different characterization techniques demonstrate
that the laser fluence can be adjusted to optimize the morphology
of the TiO2 film by increasing the contribution from volume
porosity, to improve its electrical properties and enhance its UV
photoresponse and ethanol-sensing characteristics at room temperature.
Furthermore, results of the UV and ethanol-sensing investigation show
that the optimized UV and ethanol sensors have good repeatability,
relatively fast response/recovery times, and excellent mechanical
flexibility.