Endogenously activated persulfate by non-thermal plasma for Cu(II)-EDTA decomplexation: Synergistic effect and mechanisms

Liu, Yue; Qu, Guangzhou; Sun, Qiuhong; Jia, Hanzhong; Wang, Tiecheng; Zhu, Lingyan

doi:10.1016/j.cej.2020.126774

Cited by 77 publications

(15 citation statements)

References 60 publications

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“…Plasma has been extensively used for surface activation and modification [ 23 , 24 , 25 ]. Reactive plasma species may create active sites or defects, introduce dopants, and graft surface functional groups on materials surfaces [ 12 , 26 , 27 ].…”

Section: Introductionmentioning

confidence: 99%

Dielectric Barrier Discharge Plasma Jet (DBDjet) Processed Reduced Graphene Oxide/Polypyrrole/Chitosan Nanocomposite Supercapacitors

et al. 2021

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Reduced graphene oxide (rGO) and/or polypyrrole (PPy) are mixed with chitosan (CS) binder materials for screen-printing supercapacitors (SCs) on arc atmospheric-pressure plasma jet (APPJ)-treated carbon cloth. The performance of gel-electrolyte rGO/CS, PPy/CS, and rGO/PPy/CS SCs processed by a dielectric barrier discharge plasma jet (DBDjet) was assessed and compared. DBDjet processing improved the hydrophilicity of these three nanocomposite electrode materials. Electrochemical measurements including electrical impedance spectroscopy (EIS), cyclic voltammetry (CV), and galvanostatic charging-discharging (GCD) were used to evaluate the performance of the three types of SCs. The Trasatti method was used to evaluate the electric-double layer capacitance (EDLC) and pseudocapacitance (PC) of the capacitance. The energy and power density of the three types of SCs were illustrated and compared using Ragone plots. Our experiments verify that, with the same weight of active materials, the combined use of rGO and PPy in SCs can significantly increase the capacitance and improve the operation stability.

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Section: Introductionmentioning

confidence: 99%

Dielectric Barrier Discharge Plasma Jet (DBDjet) Processed Reduced Graphene Oxide/Polypyrrole/Chitosan Nanocomposite Supercapacitors

et al. 2021

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“…[23] Besides, there is a peak at 532 cm À 1 , which is characteristic for CuÀ N/O. [24,25] For the FT-IR spectrum of the Cu catalyst, the characteristic absorptions of BmimNO 3 are absent (Figure 2a). The…”

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confidence: 99%

Anchoring Ionic Liquid in Copper Electrocatalyst for Improving CO₂ Conversion to Ethylene

et al. 2022

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Electrochemical conversion of CO 2 to valuable fuels is appealing for CO 2 fixation and energy storage. The Cu-based catalysts feature unique superiorities, but achieving high ethylene selectivity is still restricted. In this study, we propose the anchoring of an ionic liquid (IL) on a Cu electrocatalyst for improving the electrochemical CO 2 reduction to ethylene. In a water-based electrolyte and a commonly used H-type cell, a high ethylene Faradaic efficiency of 77.3 % was achieved at À 1.49 V (vs. RHE). Experimental and theoretical studies reveal that an IL can modify the electronic structure of a Cu catalyst through its interaction with Cu, making it more conducive to *CO dimerization for ethylene formation.

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“…The contents of ROS were positively related to the plasma intensity. 48 At 11 kV, the elimination efficiencies of integron intI1, aac(3)-II, blaTEM-1, tetW, and tetC reached the highest values of 4.46, 5.51, 4.77, 2.38, and 2.04 log after 10 min inactivation, respectively. DNA strand breaks, DNA− DNA intrastrand adducts, abasic sites, and bases of DNA could be oxidized by • OH.…”

Section: Resultsmentioning

confidence: 90%

Insights into DNA Structures during Antibiotic-Resistance Gene Elimination by Mesoporous Plasma

Song

Wang

et al. 2021

ACS EST Water

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The prevalence of various antibiotic-resistant bacteria (ARB) and antibiotic-resistance genes (ARGs) is becoming a global environmental problem. Removal of multiple resistant Escherichia coli strains, carrying a gentamicin resistance gene (aac(3)-II), an amoxicillin-resistance gene (blaTEM-1), tetracycline-resistance genes (tetC and tetW), and integron gene intI1, was investigated using a mesoporous plasma. The experimental results showed that the elimination efficiencies of integron intI1, aac(3)-II, blaTEM-1, tetW, and tetC reached 5.46, 5.71, 5.19, 2.88, and 2.28 log within 10 min of plasma oxidation, respectively. These elimination performances were positively related to the plasma intensity, duration time, and airflow rate. The cell membrane structures were significantly destroyed by the plasma oxidation, accompanied by leakage of ARG-containing DNA. Most of the ARG-containing DNA (more than 96%) was effectively damaged and decomposed to cytosine, guanine, adenine, and thymine. The present research revealed the removal behaviors of ARGs by plasma oxidation and provided an alternative to eliminate ARGs in an aqueous system.

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Endogenously activated persulfate by non-thermal plasma for Cu(II)-EDTA decomplexation: Synergistic effect and mechanisms

Cited by 77 publications

References 60 publications

Dielectric Barrier Discharge Plasma Jet (DBDjet) Processed Reduced Graphene Oxide/Polypyrrole/Chitosan Nanocomposite Supercapacitors

Dielectric Barrier Discharge Plasma Jet (DBDjet) Processed Reduced Graphene Oxide/Polypyrrole/Chitosan Nanocomposite Supercapacitors

Anchoring Ionic Liquid in Copper Electrocatalyst for Improving CO₂ Conversion to Ethylene

Insights into DNA Structures during Antibiotic-Resistance Gene Elimination by Mesoporous Plasma

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Endogenously activated persulfate by non-thermal plasma for Cu(II)-EDTA decomplexation: Synergistic effect and mechanisms

Cited by 77 publications

References 60 publications

Dielectric Barrier Discharge Plasma Jet (DBDjet) Processed Reduced Graphene Oxide/Polypyrrole/Chitosan Nanocomposite Supercapacitors

Dielectric Barrier Discharge Plasma Jet (DBDjet) Processed Reduced Graphene Oxide/Polypyrrole/Chitosan Nanocomposite Supercapacitors

Anchoring Ionic Liquid in Copper Electrocatalyst for Improving CO2 Conversion to Ethylene

Insights into DNA Structures during Antibiotic-Resistance Gene Elimination by Mesoporous Plasma

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Product

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Anchoring Ionic Liquid in Copper Electrocatalyst for Improving CO₂ Conversion to Ethylene