Ternary AlInN alloys are viewed as useful component materials for GaN-based electronic and optical devices, such as barrier layers in heterostructure field-effect transistors (HFETs), [1,2] or cladding layers, [3,4] distributed Bragg reflectors (DBRs), [5,6] and active layers [7,8] in light-emitting devices. For the past several years, we have conducted intensive research on the epitaxial growth and characterization of c-plane AlInN layers with thicknesses of around 300 nm using metal-organic chemical vapor deposition (MOCVD), [9][10][11][12][13][14][15][16][17][18] as primarily aiming at their application to cladding layers in GaN-based visible laser diodes (LDs). Through those studies, we found the following thing.