“…Regarding the materials used, various crystals have been explored for THz DFG, starting with simple bulk configurations in inorganic materials, such as lithium niobate (LiNbO 3 ) [74,75], lithium tantalate (LiTaO 3 ) [75,76], zinc telluride (ZnTe) [77,78], indium phosphide (InP) [79], gallium arsenide (GaAs) [80], gallium selenide (GaSe) [81,82], cadmium telluride (CdTe) [83], cadmium zinc telluride (CdZnTe) [84], and gallium phosphide (GaP) [85]. The main limitation of these sources relies on the low power achieved, due to the low efficiency of the second-order phenomenon implied in the generation.…”