technologies are attracting considerable attention owing to the increasing demand for multiplexed signal processing of broad band stimulation for accurate recognition. Recently, the development of photode tectors such as photodiodes, [11][12][13] photo conductors, [14,15] phototransistors, [16][17][18][19] and photovoltaics [20][21][22] has promoted research to enhance efficiency and sensitivity with multispectral imaging availability for the UV, [23][24][25] visible, [26,27] and IR [28][29][30][31] wave band analysis. In particular, epitaxial semiconductors such as complementary metaloxidesemiconductors (CMOS) compatible silicon technologies have led to revolutionary improvements in sen sory devices because of reasonable cost, large area, and highresolution imaging applicability. [3,32,33] However, their lim ited sensing and actuation functionalities limit opportunities for the realization of multifunctional and multiplexed stateof theart optoelectronics. Furthermore, the difficulty of integrating silicon and III-V semiconductors with printable and flexible platforms has prevented implementation in mechanically com pliant and conformal systems.As an alternative approach to epitaxially grown semiconduc tors, colloidal quantum dots (QDs) have been widely inves tigated as semiconductor nanocrystals for various optoelec tronic applications such as photodetectors, [34,35] lightemitting Color-selective multifunctional and multiplexed photodetectors have attracted considerable interest with the increasing demand for color filter-free optoelectronics which can simultaneously process multispectral signal via minimized system complexity. The low efficiency of color-filter technology and conventional laterally pixelated photodetector array structures often limit opportunities for widespread realization of high-density photodetectors. Here, low-temperature solution-processed vertically stacked full color quantum dot (QD) phototransistor arrays are developed on plastic substrates for highresolution color-selective photosensor applications. Particularly, the three different-sized/color (RGB) QDs are vertically stacked and pixelated via direct photopatterning using a unique chelating chalcometallate ligand functioning both as solubilizing component and, after photoexposure, a semiconducting cement creating robust, insoluble, and charge-efficient QD layers localized in the a-IGZO transistor region, resulting in efficient wavelength-dependent photo-induced charge transfer. Thus, high-resolution vertically stacked full color QD photodetector arrays are successfully implemented with the density of 5500 devices cm -2 on ultrathin flexible polymeric substrates with highly photosensitive characteristics such as photoresponsivity (1.1 × 10 4 AW -1 ) and photodetectivity (1.1 × 10 18 Jones) as well as wide dynamic ranges (>150 dB).