a b s t r a c t a r t i c l e i n f oDielectric elastomers (DEs) are being exploited for biological applications such as artificial blood pumps, biomimetic grippers and biomimetic robots. Generally, polyacrylate and silicone rubber (SR) are the most widely used materials for fabricating DEs in terms of mixing with other polymers or compounding them with highly dielectric particles. Furthermore, pre-stretch offers an effective approach to increasing actuated strain and dielectric strength and eliminating 'pull-in' instability. In the work described here, a comparison in electromechanical properties was made between SR/10% barium titanate (BaTiO 3 ) and commercial VHB 4910. Trends in these dielectric parameters are shown graphically for variation in pre-stretch ratio (λ pre ). It was found that permittivity of SR/10% BaTiO 3 was independent of frequency, whereas permittivity was frequency-independent due to the polarization of polymer chains. The maximum deformation and the coupling efficiency for SR/10% BaTiO 3 can be achieved at a pre-stretch ratio between 1.6 and 1.9. For VHB 4910, they can be obtained in the prestretch ratio range from 2.6 to 3.0. A maximum energy density of 0.05 MJ/m 3 was achieved by SR/10% BaTiO 3 (λ pre = 1.6) and VHB 4910 (λ pre = 3.4). The findings provide an insight into critical pre-stretch ratios required for a range of applications of DEs based on silicone and the commercially available polyacrylate VHB 4910.