2021
DOI: 10.4209/aaqr.2020.05.0193
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Effect of Boundary Layer Evolution on Nitrogen Dioxide (NO2) and Formaldehyde (HCHO) Concentrations at a High-altitude Observatory in Western India

Abstract: Highlights  We report the first simultaneous observations nitrogen dioxide (NO2) and formaldehyde (HCHO) at a high altitude station in the Western Ghats region of India.  Both NO2 and HCHO show an increasing trend throughout the day unlike a photochemistry dominated profile.  We conclude that boundary layer evolution controls the diurnal profiles of these trace gases at this high altitude site in Western India.

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Cited by 5 publications
(4 citation statements)
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References 40 publications
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“…Satellite-recorded formaldehyde concentrations take into account the entire atmospheric column from the ground to the sensor-which, in the case of TROPOMI, is at an altitude of 824 km. However, HCHO is a short-lived constituent that remains below the planetary boundary layer (up to 3 km), with higher concentrations near the surface [26,28]. In order to make it possible to compare the concentrations monitored by TROPOMI and those monitored by surface stations, presented by other works [37,[63][64][65], a methodology was proposed to estimate the surface formaldehyde concentration in the MASP, converting the data in mol/m² to ppbv.…”
Section: Estimate Of Hcho Surface Concentrationmentioning
confidence: 99%
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“…Satellite-recorded formaldehyde concentrations take into account the entire atmospheric column from the ground to the sensor-which, in the case of TROPOMI, is at an altitude of 824 km. However, HCHO is a short-lived constituent that remains below the planetary boundary layer (up to 3 km), with higher concentrations near the surface [26,28]. In order to make it possible to compare the concentrations monitored by TROPOMI and those monitored by surface stations, presented by other works [37,[63][64][65], a methodology was proposed to estimate the surface formaldehyde concentration in the MASP, converting the data in mol/m² to ppbv.…”
Section: Estimate Of Hcho Surface Concentrationmentioning
confidence: 99%
“…This is a problem for the remote monitoring of tropospheric ozone, since the highest concentrations of O 3 are found in the stratosphere, requiring the use of algorithms that make estimates based on the collected data [27]. However, because of its lifetime of a few hours, formaldehyde remains close to the surface, below the planetary boundary layer [28], which increases the reliability of the data and allows inferences to be made about its VOC precursors that also have a short lifetime (thus, they are oxidized and produce formaldehyde near the location where they were emitted) [29][30][31], on the photochemical activity of the atmosphere [32,33] and on tropospheric ozone concentrations, improving the aforementioned algorithms [27].…”
Section: Introductionmentioning
confidence: 99%
“…Among the pollutants of motor vehicle exhaust, CO makes the largest contribution to motor vehicle exhaust. NO2 is the most toxic of the NOx and can form photochemical smog (Zamorategui-Molina et al, 2021;Biswas et al, 2021;Liu et al, 2022). These harmful gases diffuse into the air will cause air pollution and harm the human body.…”
Section: Introductionmentioning
confidence: 99%
“…As concentrações de formaldeído registradas por satélite levam em consideração toda a coluna atmosférica, desde o solo até o sensorque, no caso do TROPOMI, está a uma altitude de 824 km. No entanto, o HCHO é um constituinte de vida curta e que se mantém abaixo da camada limite planetária (até 3 km), com concentrações maiores próximo à superfície (BISWAS et al, 2021;SCHROEDER et al, 2016). De modo a possibilitar a comparação entre as concentrações monitoraradas pelo TROPOMI e as monitoradas por estações em superfície, apresentadas por outros trabalhos, propôs-se uma metodologia para estimar a concentração em superfície, convertendo os dados em 10 -4 mol/m² para Considerando as alturas médias para cada mês, a metodologia proposta considera que todo o formaldeído registrado em uma coluna atmosférica se encontra homogeneamente distribuído abaixo da CLP.…”
Section: Estimativa Da Concentração Em Superfícieunclassified