“…Meanwhile, the carbon-based conductive fillers, with a sufficient mechanical property as well as light weight, are broadly applied in piezoresistive sensors, possessing a tremendous potential in pressure-response displays, animal movement detecting, healthcare monitoring, etc . , Therefore, microscale carbon-based fillers, e.g ., graphene, carbon black, or carbon fibers, become a preferred choice for future high-performance and mass-manufactured soft tactile sensors . Recently, these piezoresistive sensors based on microscale carbon-based fillers have mainly been demonstrated by two strategies as follows: first, the porous conductive active layer (hollow spherical structure or sponges); second, bionic microstructures (fish-scale-like sensing layer, cracks, interlocking, and pyramid). − Although these structures contribute to sensing sensitivity, the sensitivity is limited by little change of resistance. − In more detail, the resistance of the device changes dominantly relies on its structural compression ratio and the interconnection of conductive pathways. And the magnitude of these resistance changes, in turn, reflects the sensitivity, which is of paramount importance for the pressure sensor.…”