“…It means that the negative effect (which initially could be expected because of the less uniform coating with the enlargement in the electrode from the typical lab-size to a pilot-scale) is not observed with this novel method of preparing the anodes. Besides, the optimized design of the cell has led to an improved behavior associated with a better fluid-dynamics, as it was stated in previous works using this novel type of cells [39].…”
Section: Synergistic Effect and Energy Consumption Assessmentmentioning
confidence: 55%
“…As a result of all reactions occurring, NaOH is accumulated (Eq. ( 13)), which is responsible for turning the medium alkaline with the time [39].…”
Section: Ionic Species and Oxidants In The Electrolysis And Photo-electrolysismentioning
“…It means that the negative effect (which initially could be expected because of the less uniform coating with the enlargement in the electrode from the typical lab-size to a pilot-scale) is not observed with this novel method of preparing the anodes. Besides, the optimized design of the cell has led to an improved behavior associated with a better fluid-dynamics, as it was stated in previous works using this novel type of cells [39].…”
Section: Synergistic Effect and Energy Consumption Assessmentmentioning
confidence: 55%
“…As a result of all reactions occurring, NaOH is accumulated (Eq. ( 13)), which is responsible for turning the medium alkaline with the time [39].…”
Section: Ionic Species and Oxidants In The Electrolysis And Photo-electrolysismentioning
“…For example, the combination of water desalination with carbon storage through ex situ CO 2 mineralization 15 has been proposed to mitigate the impact of the technology and increase its sustainability. [225][226][227] Indeed, the waste brine generated through desalination is a potential source for CO 2 mineralization, because in brine the concentration of divalent cations (i.e., Ca 2+ and Mg 2+ ) necessary for binding CO 2 into stable minerals, is almost twice that of ordinary seawater. For instance, the process proposed by Oh et al (2018) 225 can achieve up to 230 tonne CO 2 reduction per year in addition to an economical benefit of water desalination.…”
Section: Ensuring Water Securitymentioning
confidence: 99%
“…[225][226][227] Indeed, the waste brine generated through desalination is a potential source for CO 2 mineralization, because in brine the concentration of divalent cations (i.e., Ca 2+ and Mg 2+ ) necessary for binding CO 2 into stable minerals, is almost twice that of ordinary seawater. For instance, the process proposed by Oh et al (2018) 225 can achieve up to 230 tonne CO 2 reduction per year in addition to an economical benefit of water desalination. However, the precipitation kinetics of carbonate minerals changes with brine composition and an intense experimental activity is required to determine the rates.…”
We describe how lab-on-a-chip systems can help address challenges in: (I) carbon sequestration, (II) hydrogen storage, (III) geothermal energy extraction, (IV) bioenergy, (V) recovering critical materials, and (VI) water filtration and remediation.
“…Concentrated CO 2 would be released with absorbent regeneration, while only partial concentrated CO 2 might be further utilized as a raw material for other industrial manufactures. CO 2 mineralization, proposed to convert gaseous CO 2 into solid carbonates with calcium or magnesium raw materials, is regarded as a potential technology to realize large-scale CO 2 fixation. , Various CO 2 mineralization technologies have been developed, including alkaline or nonalkaline ore or industry waste. − Due to physical or chemical stability of the ore or industry waste, the mineralization rate of direct exploitation is low. The raw materials should be usually activated at first. − …”
Integrated CO 2 absorption and mineralization (IAM) is a promising approach to fix CO 2 in a far less energyintensive way. The semidry flue gas desulfurization (SFGD) slag containing a considerable amount of Ca(OH) 2 is potential for mineralizing CO 2 . In this work, an IAM process combining monoethanolamine (MEA)-based CO 2 absorption and mineralization with SFGD slag is proposed and investigated to provide a systematical evaluation of the net CO 2 fixation. A desorption efficiency of 68% and an entrainment efficiency of 32 wt % were experimentally determined. An entire IAM process model with a design specification of 8350 N m 3 /h flue gas feeding and a CO 2 fixation efficiency of 90% is simulated using Aspen Plus software. Net CO 2 fixation efficiency is analyzed through life-cycle assessment (LCA). A direct relationship between parameters and LCA of CO 2 emission is built based on parameter sensitivity analysis. The IAM process, achieving the goal of gaseous waste treatment with solid waste, shows significant environmental benefits in reducing CO 2 emission. MEA loss is the major contributor to CO 2 emission, and energy consumption follows. A net CO 2 fixation efficiency of 87.6% can be obtained with the optimized parameters. Reducing MEA loss would be effective to increase net CO 2 fixation efficiency of the whole process. This work provides a quantitative understanding of CO 2 fixation of the IAM process for industrial application and a guideline for further process optimization.
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