“…Since its initial demonstration in 2012, triboelectric nanogenerators (TENGs) that can effectively harvest environmental mechanical energy have been the subject of intense research. − It has a high power output, an adaptable structural design, and a variety of material choices. Development of the TENGs has spawned a slew of new uses, such as flexible electronics, wireless sensing, catalysis, medicine, and other fields. − Meanwhile, the choice of the tribolayer material for TENGs presents tougher challenge when trying to get a higher electrical output. − While traditional polymers provide a considerable electrical output for TENGs, the environmental pollution caused by their nondegradable properties is inevitable. − Bio-based materials have become important materials for the preparation of electropositive tribolayers of TENGs due to their wide sources, degradability, and simple preparation. Among them, cellulose nanofibers (CNFs) with excellent mechanical properties and transparency have gained increasing attention. − CNFs can guide TENGs toward a more environmentally conscious system that is also naturally biocompatible, recyclable, and degradable.…”